Possible excitonic insulating phase in quantum-confined Sb nanoflakes
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Date
2019-07-10
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American Chemical Society
Abstract
In the 1960s, it was proposed that in small indirect band-gap materials, excitons can spontaneously form because the density of carriers is too low to screen the attractive Coulomb interaction between electrons and holes. The result is a novel strongly interacting insulating phase known as an excitonic insulator. Here we employ scanning tunnelling microscopy (STM) and spectroscopy (STS) to show that the enhanced Coulomb interaction in quantum-confined elemental Sb nanoflakes drives the system to the excitonic insulator state. The unique feature of the excitonic insulator, a charge density wave (CDW) without periodic lattice distortion, is directly observed. Furthermore, STS shows a gap induced by the CDW near the Fermi surface. Our observations suggest that the Sb(110) nanoflake is an excitonic insulator. © 2019 American Chemical Society.
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Keywords
Antimony, Excitons, Coulomb field, Electrical insulators, Quantum computers, Nanoparticles, Microscopy, Spectroscopy, Electrons
Citation
Li, Z., Nadeem, M., Yue, Z., Cortie, D., Fuhrer, M., & Wang, X. (2019). Possible excitonic insulating phase in quantum-confined Sb nanoflakes. Nano letters, 19(8), 4960-4964. doi:10.1021/acs.nanolett.9b01123