ANSTO Publications Online

Welcome to the ANSTO Institutional Repository known as APO.

The APO database has been migrated to version 7.5. The functionality has changed, but the content remains the same.

ANSTO Publications Online is a digital repository for publications authored by ANSTO staff since 2007. The Repository also contains ANSTO Publications, such as Reports and Promotional Material. ANSTO publications prior to 2007 continue to be added progressively as they are in identified in the library. ANSTO authors can be identified under a single point of entry within the database. The citation is as it appears on the item, even with incorrect spelling, which is marked by (sic) or with additional notes in the description field.

If items are only held in hardcopy in the ANSTO Library collection notes are being added to the item to identify the Dewey Call number: as DDC followed by the number.

APO will be integrated with the Research Information System which is currently being implemented at ANSTO. The flow on effect will be permission to publish, which should allow pre-prints and post prints to be added where content is locked behind a paywall. To determine which version can be added to APO authors should check Sherpa Romeo. ANSTO research is increasingly being published in open access due mainly to the Council of Australian University Librarians read and publish agreements, and some direct publisher agreements with our organisation. In addition, open access items are also facilitated through collaboration and open access agreements with overseas authors such as Plan S.

ANSTO authors are encouraged to use a CC-BY licence when publishing open access. Statistics have been returned to the database and are now visible to users to show item usage and where this usage is coming from.

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The impact of fire on the geochemistry of speleothem-forming drip water in a sub-alpine cave
(Elsevier, 2018-11) Coleborn, K; Baker, AA; Treble, Pauline C; Andersen, MS; Baker, AC; Tadros, CV; Tozer, MG; Fairchild, IJ; Spate, A; Meehan, S
Fire dramatically modifies the surface environment by combusting vegetation and changing soil properties. Despite this well-documented impact on the surface environment, there has been limited research into the impact of fire events on karst, caves and speleothems. Here we report the first experiment designed to investigate the short-term impacts of a prescribed fire on speleothem-forming cave drip water geochemistry. Before and after the fire, water was collected on a bi-monthly basis from 18 drip sites in South Glory Cave, New South Wales, Australia. Two months post-fire, there was an increase in B, Si, Na, Fe and Pb concentrations at all drip sites. We conclude that this response is most likely due to the transport of soluble ash-derived elements from the surface to the cave drip water below. A significant deviation in stable water isotopic composition from the local meteoric water line was also observed at six of the sites. We hypothesise that this was due to partial evaporation of soil water resulting in isotopic enrichment of drip waters. Our results demonstrate that even low-severity prescribed fires can have an impact on speleothem-forming cave drip water geochemistry. These findings are significant because firstly, fires need to be considered when interpreting past climate from speleothem δ18O isotope and trace element records, particularly in fire prone regions such as Australia, North America, south west Europe, Russia and China. Secondly, it supports research that demonstrates speleothems could be potential proxy records for past fires. © 2018 Elsevier B.V.
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Formation and characteristics of ions and charged aerosol particles in a native Australian Eucalypt forest
(Copernicus Publications, 2008-01-14) Suni, T; Kulmala, M; Hirsikko, A; Bergman, T; Laakso, L; Aalto, PP; Leuning, R; Cleugh, H; Zegelin, S; Hughes, D; van Gorsel, E; Kitchen, M; Vana, M; Hõrrak, U; Mirme, S; Mirme, A; Sevanto, S; Twining, JR; Tadros, CV
Abstract. Biogenic aerosol formation is likely to contribute significantly to the global aerosol load. In recent years, new-particle formation has been observed in various ecosystems around the world but hardly any measurements have taken place in the terrestrial Southern Hemisphere. Here, we report the first results of atmospheric ion and charged particle concentrations as well as of new-particle formation in a Eucalypt forest in Tumbarumba, South-East Australia, from July 2005 to October 2006. The measurements were carried out with an Air Ion Spectrometer (AIS) with a size range from 0.34 to 40 nm. The Eucalypt forest was a very strong source of new aerosol particles. Daytime aerosol formation took place on 52% of days with acceptable data, which is 2–3 times as often as in the Nordic boreal zone. Average growth rates for negative/positive 1.5–3 nm particles during these formation events were 2.89/2.68 nmh−1, respectively; for 3-7 nm particles 4.26/4.03, and for 7–20 nm particles 8.90/7.58 nmh−1, respectively. The growth rates for large ions were highest when the air was coming from the native forest which suggests that the Eucalypts were a strong source of condensable vapours. Average concentrations of cluster ions (0.34–1.8 nm) were 2400/1700 cm−3 for negative/positive ions, very high compared to most other measurements around the world. One reason behind these high concentrations could be the strong radon efflux from the soils around the Tumbarumba field site. Furthermore, comparison between night-time and daytime concentrations supported the view that cluster ions are produced close to the surface within the boundary layer also at night but that large ions are mostly produced in daytime. Finally, a previously unreported phenomenon, nocturnal aerosol formation, appeared in 32% of the analysed nights but was clustered almost entirely within six months from summer to autumn in 2006. From January to May, nocturnal formation was 2.5 times as frequent as daytime formation. Therefore, it appears that in summer and autumn, nocturnal production was the major mechanism for aerosol formation in Tumbarumba. © Author(s) 2008. This work is licensed under the Creative Commons Attribution-NonCommercial-Share Alike 2.5 Licence.
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Cave drip water solutes in south-eastern Australia: constraining sources, sinks and processes
(Elsevier, 2019-02-15) Tadros, CV; Treble, PC; Baker, AA; Hankin, SI; Roach, R
Constraining sources and site-specific processes of trace elements in speleothem geochemical records is key to an informed interpretation. This paper examines a 10-year data set of drip water solutes from Harrie Wood Cave, south-eastern Australia, and identifies the processes that control their response to El Niño-Southern Oscillation events which varies the site water balance. The contributions of aerosol and bedrock end-members are quantified via hydrochemical mass balance modelling. The parent bedrock is the main source for the drip water solutes: Mg, Sr, K and trace elements (Ba, Al, V, Cr, Mn, Ni, Co, Cu, Pb and U), while atmospheric aerosol inputs also contribute significantly to drip water trace elements and Na, K and Zn. A laboratory investigation evaluating water-soluble fractions of metals in soil samples and soil enrichment factors provided a basis for understanding metal retainment and release to solution and transport from the soil zone. These results identified the role of the soil as a sink for: trace metals, Na and K, and a secondary source for Zn. Further, soil processes including: cation exchange, K-fixation, metal adsorption to colloids and the release of Zn associated with organic matter degradation further modify the chemical composition of the resultant drip waters. This research is significant for the south-eastern Australian region, as well as other sites in a karst setting with clay-rich soil. In particular these results reveal that the response of drip water chemistry to hydroclimatic forcing is non-linear, with the greatest response observed when the long-term gradient in the cumulative water balance reverses. This longer-term drip water monitoring dataset is significant because it provides the pivotal framework required to reliably identify suitable trace element proxies for interpretation in geochemical speleothem records on multi-decadal timescales. © 2018 Crown Copyright © 2018 Published by Elsevier B.V.
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Parameters controlling emission of terahertz frequency electromagnetic radiation from InAs and GaAs: an ensemble Monte Carlo simulation study
(The Electrochemical Society, 2013-03-15) Cortie, DL; Lewis, RA
The generation, manipulation and detection of terahertz-frequency electromagnetic radiation are topics of great current theoretical and experimental interest. In particular, the coherent generation and detection of ultrashort pulses of terahertz radiation has opened up the field of terahertz time-domain spectroscopy, which permits the simultaneous measurement of amplitude and phase of the terahertz electric field. In this paper, the emission of terahertz radiation from bare semiconductor surfaces following photoexcitation by ultrashort pulses of near-infrared radiation is studied using ensemble Monte Carlo simulations. The simulation allows us to examine separately distinct scattering mechanisms and to vary the materials parameters of bandgap, absorption coefficient, effective mass, and surface potential. The narrower-gap semiconductor InAs and the wider-gap semiconductor GaAs are given as examples in which diffusion and drift processes, respectively, dominate. We find that scattering is relatively unimportant in the case of InAs but is very important in the case of GaAs. © The Electrochemical Society
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8Li+ β-NMR in the cubic insulator MgO
(IOP Publishing, 2014-12-16) MacFarlane, WA; Parolin, TJ; Cortie, DL; Chow, KH; Hossain, MD; Kiefl, RF; Levy, CDP; McFadden, RML; Morris, GD; Pearson, MR; Saadaoui, H; Salman, Z; Song, Q; Wang, D
We present extensive high magnetic field β-NMR measurements of 8Li+ implanted in single crystals of MgO. The narrow resonance, consistent with a cubic 8Li+ site, likely the tetrahedral interstitital, is used routinely as a reference for shift measurements. We show the intrinsic linewidth is on the order of 200 Hz, allowing a frequency determination to an accuracy of a few Hz. We find no implantation energy dependence of the resonance within a few ppm, but there is evidence of slow spin dynamics in hole-burning measurements. The spin lattice relaxation is slow. The temperature dependence reveals interesting changes at low temperature whose origin remains uncertain. Open Access CC-BY