The promise of high-entropy materials for high-performance rechargeable Li-ion and Na-ion batteries

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dc.contributor.authorZheng, Wen_AU
dc.contributor.authorLiang, Gen_AU
dc.contributor.authorLiu, Qen_AU
dc.contributor.authorLi, JXen_AU
dc.contributor.authorYuwono, JAen_AU
dc.contributor.authorZhang, Sen_AU
dc.contributor.authorPeterson, VKen_AU
dc.contributor.authorGuo, ZPen_AU
dc.date.accessioned2025-01-09T02:48:44Zen_AU
dc.date.available2025-01-09T02:48:44Zen_AU
dc.date.issued2023-12-20en_AU
dc.date.statistics2024-11-26en_AU
dc.descriptionW.Z. gratefully acknowledges the support of the China Scholarship Council (No. 202108430035). This work is supported by the Australian Research Council under grants DP200101862, DP210101486, and FL210100050.en_AU
dc.description.abstractOur growing dependence on rechargeable Li/Na-ion batteries calls for substantial improvements in the electrochemical performance of battery materials, including cathodes, anodes, and electrolytes. However, the performance enhancements based on traditional modification methods of elemental doping and surface coating are still far from the target of high-performance rechargeable batteries. Fortunately, the recent emergence of high-entropy materials preserving a stable solid-state phase for energy-related applications provides unprecedented flexibility and variability in materials composition and electronic structure, opening new avenues to accelerate battery materials development. This perspective first presents clear qualitative and quantitative definitions for high-entropy battery materials, as well as summarizes the enhancement mechanisms. Then, we comprehensively review state-of-the-art research progress and highlight key factors in the rational design of advanced high-entropy battery materials from both experimental and calculational aspects. Moreover, the challenges limiting the progress of this research are presented, alongside insights and approaches to address these issues at the research forefront. Finally, we outline potential directions for extending the future development of the high-entropy strategy to solve other critical issues in battery materials research. This perspective will guide researchers in their studies toward the development of high-performance rechargeable Li-ion and Na-ion batteries. © 2024 Elsevier Inc. - Open Archiveen_AU
dc.identifier.citationZheng, W., Liang, G., Liu, Q., Li, J., Yuwono, J. A., Zhang, S., Peterson, V. K., & Guo, Z. (2023). The promise of high-entropy materials for high-performance rechargeable Li-ion and Na-ion batteries. Joule, 7(12), 2732-2748. doi:10.1016/j.joule.2023.10.016en_AU
dc.identifier.issn2542-4785en_AU
dc.identifier.issn2542-4351en_AU
dc.identifier.issue12en_AU
dc.identifier.journaltitleJouleen_AU
dc.identifier.pagination2732-2748en_AU
dc.identifier.urihttps://doi.org/10.1016/j.joule.2023.10.016en_AU
dc.identifier.urihttps://apo.ansto.gov.au/handle/10238/15863en_AU
dc.identifier.volume7en_AU
dc.languageEnglishen_AU
dc.language.isoenen_AU
dc.publisherElsevieren_AU
dc.subjectEntropyen_AU
dc.subjectSodiumen_AU
dc.subjectLithiumen_AU
dc.subjectLithium ion batteriesen_AU
dc.subjectPerformanceen_AU
dc.subjectCathodesen_AU
dc.subjectAnodesen_AU
dc.subjectElectrolytesen_AU
dc.subjectMaterialsen_AU
dc.subjectMetal-metal Oxide batteriesen_AU
dc.titleThe promise of high-entropy materials for high-performance rechargeable Li-ion and Na-ion batteriesen_AU
dc.typeJournal Articleen_AU
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