Ice core measurements of 14CH4 constrain the sources of atmospheric methane increase during abrupt warming events of the last deglaciation

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dc.contributor.authorPetrenko, VVen_AU
dc.contributor.authorSeveringhaus, JPen_AU
dc.contributor.authorSmith, AMen_AU
dc.contributor.authorRiedel, Ken_AU
dc.contributor.authorBrook, EJen_AU
dc.contributor.authorSchaefer, Hen_AU
dc.contributor.authorBaggenstos, Den_AU
dc.contributor.authorHarth, CMen_AU
dc.contributor.authorHua, Qen_AU
dc.contributor.authorDyonisius, MNen_AU
dc.contributor.authorBuizert, Cen_AU
dc.contributor.authorSchilt, Aen_AU
dc.contributor.authorFaïn, Xen_AU
dc.contributor.authorMitchell, Len_AU
dc.contributor.authorBauska, TKen_AU
dc.contributor.authorOrsi, AJen_AU
dc.contributor.authorWeiss, RFen_AU
dc.date.accessioned2020-05-18T06:25:39Zen_AU
dc.date.available2020-05-18T06:25:39Zen_AU
dc.date.issued2015-12-01en_AU
dc.date.statistics2020-05-18en_AU
dc.description.abstractThawing permafrost and marine methane hydrate destabilization in the Arctic and elsewhere have been proposed as large sources of methane to the atmosphere in the future warming world. To evaluate this hypothesis it is useful to ask whether such methane releases happened during past warming events. The two major abrupt warming events of the last deglaciation, Oldest Dryas - Bølling (OD-B, ≈ 14,500 years ago) and Younger Dryas - Preboreal (YD-PB; ≈11,600 years ago), were associated with large (up to 50%) increases in atmospheric methane (CH4) concentrations. The sources of these large warming-driven CH4 increases remain incompletely understood, with possible contributions from tropical and boreal wetlands, thawing permafrost as well as marine CH4 hydrates. We present a record of 14C of paleoatmospheric CH4 over the YD-PB transition from ancient ice outcropping at Taylor Glacier, Antarctica. 14C can unambiguously identify CH4 emissions from old, 14C-depleted sources, such as permafrost and CH4 hydrates. The only prior study of paleoatmospheric 14CH4 (from Greenland ice) suggested that wetlands were the main driver of the YD-PB CH4 increase, but the results were weakened by an unexpected and poorly understood 14CH4 component from in situ cosmogenic production directly in near-surface ice. In this new study, we have been able to accurately characterize and correct for the cosmogenic 14CH4 component. All samples from before, during and after the abrupt warming and associated CH4 increase yielded 14CH4 values that are consistent with 14C of atmospheric CO2 at that time, indicating a purely contemporaneous methane source. These measurements rule out the possibility of large CH4 releases to the atmosphere from methane hydrates or old permafrost carbon in response to the large and rapid YD-PB warming. To the extent that the characteristics of the YD-PB warming are comparable to those of the current anthropogenic warming, our measurements suggest that large future atmospheric methane increases from old carbon sources in the Arctic are unlikely. Instead, our measurements indicate that global wetlands will likely respond to the warming with increased methane emissions. Analysis and interpretation of 14CH4 for the abrupt OD - B transition is in progress and these results will also be presented. © AGUen_AU
dc.identifier.citationPetrenko, V.V., Severinghaus, J.P., Smith A.M., Riedel, K., Brook, E., Schaefer, H., Baggenstos, D., Harth, C. M., Hua, Q., Dyonisius, M., Buizert, C., Schilt, A., Faïn, X., Mitchell, L., Bauska, T. K., Orsi, A. J., & Weiss, R. F. (2015). Ice core measurements of 14CH4 constrain the sources of atmospheric methane increase during abrupt warming events of the last deglaciation. Presentation to the American Geophysical Union, Fall Meeting, 14-18 December 2015, San Francisco.en_AU
dc.identifier.conferenceenddate18 December 2015en_AU
dc.identifier.conferencenameAmerican Geophysical Union, Fall Meetingen_AU
dc.identifier.conferenceplaceSan Francisco, Californiaen_AU
dc.identifier.conferencestartdate14 December 2015en_AU
dc.identifier.govdoc9498en_AU
dc.identifier.otherA23J-01en_AU
dc.identifier.urihttps://agu.confex.com/agu/fm15/meetingapp.cgi/Paper/75126en_AU
dc.identifier.urihttp://apo.ansto.gov.au/dspace/handle/10238/9457en_AU
dc.language.isoenen_AU
dc.publisherADSen_AU
dc.subjectEnvironmental transporten_AU
dc.subjectAtmospheric chemistryen_AU
dc.subjectBiosphereen_AU
dc.subjectTroposphereen_AU
dc.subjectGasesen_AU
dc.subjectDrill coresen_AU
dc.titleIce core measurements of 14CH4 constrain the sources of atmospheric methane increase during abrupt warming events of the last deglaciationen_AU
dc.typeConference Abstracten_AU
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