Use of accelerator mass spectrometry (AMS) to study the migration and bioaccumulation of actinides in the environment

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dc.contributor.authorHotchkis, MACen_AU
dc.contributor.authorChild, DPen_AU
dc.contributor.authorPayne, TEen_AU
dc.contributor.authorJohansen, MPen_AU
dc.contributor.authorDavis, Een_AU
dc.contributor.authorHarrison, JJen_AU
dc.contributor.authorThiruvoth, Sen_AU
dc.contributor.authorWilsher, WLen_AU
dc.date.accessioned2017-02-16T06:04:20Zen_AU
dc.date.available2017-02-16T06:04:20Zen_AU
dc.date.issued2014en_AU
dc.date.statistics2017-02-16en_AU
dc.description.abstractThe high sensitivity of AMS for actinides analysis can facilitate a range of studies aimed at improving understanding of how actinides behave in the environment. Former nuclear sites, which contain a range of levels of contamination with actinides, offer opportunities to study the migration and bioaccumulation of actinides. In addition to the evaluation of the radiological risk posed to potential human and non-human occupants of those specific sites, such studies can contribute fundamental data to the understanding of the behaviour of actinides in the environment. The Little Forest Burial Ground, located on the edge of Sydney, was used by the Australian Atomic Energy Commission to dispose of low level radioactive waste in shallow trenches in the 1960s. The waste included small amounts of uranium and plutonium with various isotopic compositions. α-spectrometry is being used as the primary method of radio-analysis in current studies of this site [1]. In addition, AMS is being applied where higher sensitivity is required, and to measure isotopes not easily measureable by α-spectrometry. 239Pu and 240Pu cannot be resolved by α-spectrometry, and 233U is poorly resolved from 234U. In both cases we can apply AMS to define these isotopic signatures. In the case of plutonium, the 240Pu/239Pu ratio can be used to distinguish local contamination sources from global fallout. The high sensitivity of AMS has enabled the detection of Pu and 233U in vegetation, providing data on uptake and bioaccumulation. The former nuclear weapons test site at Maralinga in South Australia was used in the 1950s and 1960s for seven nuclear weapon detonations and also numerous ‘safety trials’ which dispersed plutonium and uranium in the environment. By analysing plutonium in wildlife and soil samples from around this site, we are able to evaluate the uptake of plutonium and its mobility, and compare present-day results with earlier studies of the site [2]. Further work is in progress examining the distribution of plutonium in the tissues of mammals and other species inhabiting the site. By exploiting the high sensitivity of AMS, non-lethal methods for investigating actinide uptake and its effects on wildlife are being developed for this work.en_AU
dc.identifier.citationHotchkis, M., Child, D., Payne, T., Johansen, M., Davis, E., Harrison, J., Thiruvoth, S., & Wilsher, K. (2014). Use of accelerator mass spectrometry (AMS) to study the migration and bioaccumulation of actinides in the environment. Presentation to the Heavy Ion Accelerator Symposium on Fundamental and Applied Science (HIAS), 30 June – 2 July 2014, Australian National University, Canberra.en_AU
dc.identifier.conferenceenddate2 July 2014en_AU
dc.identifier.conferencenameHeavy Ion Accelerator Symposium on Fundamental and Applied Science (HIAS)en_AU
dc.identifier.conferenceplaceCanberra, Australiaen_AU
dc.identifier.conferencestartdate30 June 2014en_AU
dc.identifier.govdoc7881en_AU
dc.identifier.urihttp://hias.anu.edu.au/2014/_files/HIAS_2014_abstract_Mike_Hotchkis.pdfen_AU
dc.identifier.urihttp://apo.ansto.gov.au/dspace/handle/10238/8309en_AU
dc.language.isoenen_AU
dc.publisherAustralian National Universityen_AU
dc.subjectActinidesen_AU
dc.subjectBiological accumulationen_AU
dc.subjectForestsen_AU
dc.subjectRadioactive wastesen_AU
dc.subjectPlutoniumen_AU
dc.subjectSpectroscopyen_AU
dc.titleUse of accelerator mass spectrometry (AMS) to study the migration and bioaccumulation of actinides in the environmenten_AU
dc.typeConference Abstracten_AU
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