Lineshape of the singlet-triplet excitations in the dimer system Sr3Cr2O8 to first order in the high-density 1/z expansion

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dc.contributor.authorJensen, Jen_AU
dc.contributor.authorQuintero-Castro, DLen_AU
dc.contributor.authorIslam, ATMNen_AU
dc.contributor.authorRule, KCen_AU
dc.contributor.authorMånsson, Men_AU
dc.contributor.authorLake, Ben_AU
dc.date.accessioned2017-04-26T01:03:07Zen_AU
dc.date.available2017-04-26T01:03:07Zen_AU
dc.date.issued2014-04-11en_AU
dc.date.statistics2016-08-29en_AU
dc.description.abstractThe Cr 5+ ions in Sr 3 Cr 2 O 8 constitute a strongly correlated spin-1/2 dimer system. Experiments show that the collective singlet-triplet excitations in this system are well defined in the zero-temperature limit, but, when heated, the inelastic neutron scattering peaks decrease rapidly in intensity and acquire a nonzero line width. When including the fluctuations to leading order in 1/z , where z is the coordination number, the diagrammatic high-density expansion is found to offer an accurate description of the singlet-triplet excitations. The theory explains not only the temperature dependencies of the intensities and line widths, but also that strong correlation causes the lineshapes to become asymmetric at temperatures comparable to the excitation energies.© 2014, American Physical Society.en_AU
dc.identifier.articlenumber134407en_AU
dc.identifier.citationJensen, J., Quintero-Castro, D. L., Islam, A., Rule, K. C., Månsson, M., & Lake, B. (2014). Lineshape of the singlet-triplet excitations in the dimer system Sr3Cr2O8 to first order in the high-density 1/z expansion. Physical Review B, 89(13), 134407. doi:10.1103/PhysRevB.89.134407en_AU
dc.identifier.govdoc7047en_AU
dc.identifier.issn1550-235Xen_AU
dc.identifier.journaltitlePhysical Review Ben_AU
dc.identifier.urihttp://dx.doi.org/10.1103/PhysRevB.89.134407en_AU
dc.identifier.urihttp://apo.ansto.gov.au/dspace/handle/10238/8623en_AU
dc.identifier.volume89en_AU
dc.language.isoenen_AU
dc.publisherPhysical Review Ben_AU
dc.subjectExperiment planningen_AU
dc.subjectNeutronsen_AU
dc.subjectTemperature zero Ken_AU
dc.subjectExcitation functionsen_AU
dc.subjectEnergyen_AU
dc.subjectDimersen_AU
dc.titleLineshape of the singlet-triplet excitations in the dimer system Sr3Cr2O8 to first order in the high-density 1/z expansionen_AU
dc.typeJournal Articleen_AU
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