A novel approach for neutron-capture studies of 235U and 238U

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dc.contributor.authorWallner, Aen_AU
dc.contributor.authorBelgya, Ten_AU
dc.contributor.authorBichler, Men_AU
dc.contributor.authorBuczak, Ken_AU
dc.contributor.authorDillmann, Ien_AU
dc.contributor.authorKäppeler, Fen_AU
dc.contributor.authorMengoni, Aen_AU
dc.contributor.authorQuinto, Fen_AU
dc.contributor.authorSteier, Pen_AU
dc.contributor.authorSzentmiklósi, Len_AU
dc.date.accessioned2012-04-17T23:00:26Zen_AU
dc.date.available2012-04-17T23:00:26Zen_AU
dc.date.issued2011-03-25en_AU
dc.date.statistics2012-04-18en_AU
dc.description.abstractImproved and highly accurate nuclear data are urgently required for the design of advanced reactor concepts. This demand holds for minor actinides but also for the main fuel materials. Existing data were measured by detection of the prompt capture γ-rays. A major difficulty in these experiments is the safe discrimination against the strong γ-background from the competing fission channel. Recent studies exhibit critical discrepancies at keV energies for both, 235U(n,γ) and 238U(n,γ) with great impact on the keff-value of fission reactors. Neutron activation with subsequent accelerator mass spectrometry (AMS) measurement of the reaction product represents an independent technique, where interference from fission is completely excluded. Within the European EFNUDAT project, new measurements were performed with the goal to determine the neutron capture cross sections of 235U and 238U via neutron irradiations at thermal (cold) and keV energies: Activations were performed with cold neutrons (Budapest Research Reactor), thermal (Atominstitut, Vienna) and with neutrons of 25 and 450 keV (Karlsruhe Institute of Technology). The produced long-lived 236U and the decay product of 239U, 239Pu were subsequently counted by AMS at the Vienna Environmental Research Accelerator (VERA). This method for measuring the neutron capture cross section has the advantages that the involved systematic uncertainties are in no way correlated with those inherent to previous techniques. Therefore, this experiment provides important and independent information for these key reactions of reactor physics with uncertainties expected below 5%. The high sensitivity of AMS requires only very small samples. New results for 235U(n,γ)236U and 238U(n,γ)239U in the energy range from thermal to 500 keV will be presented. The challenges of measuring 236U/238U isotope ratios at the 10-12 level and to quantify 239Pu with high precision will be highlighted. Finally, the potential for extending that method to other isotopes in that mass range will be discussed. Copyright (c) 2011 AMS12en_AU
dc.identifier.citationWallner, A., Belgya, T., Bichler, M., Buczak, K., Dillmann, I., Käppeler, F., 4, Mengoni, A., Quinto, F., Steier, P., & Szentmiklósi, L. (2011). A novel approach for neutron-capture studies of 235U and 238U. Presentation to the 12th International Conference on Accelerator Mass Spectrometry (AMS 12), 20th - 25th March 2011. Museum of New Zealand: Te Papa Tongarewa, Wellington, New Zealand.en_AU
dc.identifier.conferenceenddate25 March 2011en_AU
dc.identifier.conferencename12th International Conference on Accelerator Mass Spectrometry (AMS 12)en_AU
dc.identifier.conferenceplaceWellington, New Zealanden_AU
dc.identifier.conferencestartdate20 March 2011en_AU
dc.identifier.govdoc4289en_AU
dc.identifier.urihttps://www.gns.cri.nz/ams12/AMS-12_Abstracts_Book_Final.pdfen_AU
dc.identifier.urihttp://apo.ansto.gov.au/dspace/handle/10238/4141en_AU
dc.language.isoenen_AU
dc.publisherGNS Scienceen_AU
dc.subjectUranium 235en_AU
dc.subjectUranium 238en_AU
dc.subjectCaptureen_AU
dc.subjectActinidesen_AU
dc.subjectAcceleratorsen_AU
dc.subjectMass spectrometersen_AU
dc.titleA novel approach for neutron-capture studies of 235U and 238Uen_AU
dc.typeConference Presentationen_AU
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