Magnetic ordering in Er2Fe2Si2C and Tm2Fe2Si2C
dc.contributor.author | Susilo, RA | en_AU |
dc.contributor.author | Cadogan, JM | en_AU |
dc.contributor.author | Hutchison, WD | en_AU |
dc.contributor.author | Campbell, SJ | en_AU |
dc.contributor.author | Avdeev, M | en_AU |
dc.contributor.author | Ryan, DH | en_AU |
dc.contributor.author | Namiki, T | en_AU |
dc.date.accessioned | 2021-08-02T22:39:43Z | en_AU |
dc.date.available | 2021-08-02T22:39:43Z | en_AU |
dc.date.issued | 2015-02 | en_AU |
dc.date.statistics | 2021-07-20 | en_AU |
dc.description.abstract | The magnetic ordering of two members of the R2Fe2Si2C (R = rare-earth) series of compounds (monoclinic Dy2Fe2Si2C-type structure with the C2/m space group), Er2Fe2Si2C and Tm2Fe2Si2C, have been studied by neutron powder diffraction and 166Er Mössbauer spectroscopy, complemented by magnetisation and specific heat measurements. In both cases, antiferromagnetic ordering of the R sublattice is observed, with Neel temperatures of 4.8(2) K and 2.6(3) K for Er2Fe2Si2C and Tm2Fe2Si2C, respectively. The magnetic structures of the Erand Tm-based compounds are quite different from those found for the other members of the R2Fe2Si2C series. Previous studies show that the common magnetic structure of the heavy- R2Fe2Si2C compounds involves ordering of the R sublattice along the b-axis with a propagation vector k = [0, 0, ½]. However, the antiferromagnetic structure of the Er sublattice in Er2Fe2Si2C is described by k = [½, ½, 0] with the Er magnetic moments lying close to the ac-plane. Tm2Fe2Si2C is found to exhibit a more complex magnetic structure that is characterised by a square-wave modulation of the Tm magnetic moments along the a-axis and a cell-doubling along the b-axis with k = [0.403(1), ½, 0]. The differences in the magnetic structures of these compounds are interpreted in terms of the RKKY exchange interaction, which depends on the R-R interatomic distances, and crystal field effects acting on the R3+ ions. | en_AU |
dc.identifier.citation | Susilo, R. A., Cadogan, J. M., Hutchison, W. D., Campbell, S. J., Avdeev, M., Ryan, D. H., & Namiki, T. (2015). Magnetic ordering in Er2Fe2Si2C and Tm2Fe2Si2C. Paper presented at 39th Annual Condensed Matter and Materials Meeting, Charles Sturt University, Wagga Wagga, NSW, 3 – 6 February 2015. Retrieved from: https://physics.org.au/wp-content/uploads/cmm/2015/Wagga2015_10_Handbook.pdf | en_AU |
dc.identifier.conferenceenddate | 6 February 2015 | en_AU |
dc.identifier.conferencename | 39th Annual Condensed Matter and Materials Meeting | en_AU |
dc.identifier.conferenceplace | Wagga Wagga, NSW | en_AU |
dc.identifier.conferencestartdate | 3 February 2015 | en_AU |
dc.identifier.isbn | 978-0-646-59459-0; | en_AU |
dc.identifier.uri | https://apo.ansto.gov.au/dspace/handle/10238/11238 | en_AU |
dc.language.iso | en | en_AU |
dc.publisher | Australian Institute of Physics | en_AU |
dc.subject | Antiferromagnetism | en_AU |
dc.subject | Thulium compounds | en_AU |
dc.subject | Crystal field | en_AU |
dc.subject | Erbium compounds | en_AU |
dc.subject | Exchange interactions | en_AU |
dc.subject | Magnetic moments | en_AU |
dc.subject | Magnetic properties | en_AU |
dc.subject | Moessbauer effect | en_AU |
dc.subject | Neel temperature | en_AU |
dc.subject | Neutron diffraction | en_AU |
dc.subject | Rare earths | en_AU |
dc.title | Magnetic ordering in Er2Fe2Si2C and Tm2Fe2Si2C | en_AU |
dc.type | Conference Abstract | en_AU |