Browsing by Author "Johnson, KR"

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    Hydrological control on the dead-carbon content of a tropical Holocene speleothem
    (Elsevier, 2012-12-01) Griffiths, ML; Fohlmeister, J; Drysdale, RN; Hua, Q; Johnson, KR; Hellstrom, JC; Gagan, MK; Zhao, JX
    Over the past decade, a number of speleothem studies have used radiocarbon (14C) to address a range of palaeoclimate problems. These have included the use of the bomb pulse 14C to anchor chronologies over the last 60 years, the combination of U-Th and 14C measurements to improve the radiocarbon age-calibration curve, and linking atmospheric 14C variations with climate change. An issue with a number of these studies is how to constrain, or interpret, variations in the amount of radioactively dead carbon (i.e. the dead carbon fraction, or DCF) that reduces radiocarbon concentrations in speleothems. In this study, we use 14C, stable-isotopes, and trace-elements in a U-Th dated speleothem from Flores, Indonesia, to examine DCF variations and their relationship with above-cave climate over the late Holocene and modern era. A strong association between the DCF and hydrologically-controlled proxy data suggests that more dead carbon was being delivered to the speleothem during periods of higher cave recharge (i.e. lower δ18O, δ13C and Mg/Ca values), and hence stronger summer monsoon. To explore this relationship, we used a geochemical soil-karst model coupled with 14C measurements through the bomb pulse to disentangle the dominant components governing DCF variability in the speleothem. We find that the DCF is primarily controlled by limestone dissolution associated with changes in open- versus closed-system conditions, rather than kinetic fractionation and/or variations in the age spectrum of soil organic matter above the cave. Therefore, we infer that periods of higher rainfall resulted in a higher DCF because the system was in a more closed state, which inhibited carbon isotope exchange between the karst water dissolved inorganic carbon and soil-gas CO2, and ultimately led to a greater contribution of dead carbon from the bedrock. © 2020 Elsevier B.V.
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    Hydrological influence on the dead carbon fraction in a tropical speleothem during the Younger Dryas and the Last Millennium
    (American Geophyical Union, 2015-11-16) Griffiths, ML; Hua, Q; Drysdale, RN; Bajo, P; Jenkins, D; Hellstrom, JC; Johnson, KR; Gagan, MK; Zhao, JX
    The number of paleoclimate records derived from speleothems has increased significantly in recent years. In addition, speleothems have been used for calibration of the radiocarbon timescale beyond the range of the tree-ring record. One critical issue for reliable speleothem-based radiocarbon calibration and 14C dating of speleothems is constraining the temporal variations in the radioactively dead carbon (i.e. dead carbon fraction (DCF)) that is incorporated into this archive and to determine the potential mechanisms driving such changes. While some studies have shown insignificant variations in DCF through time and highlighted the potential utility of speleothems to extend/improve the radiocarbon calibration curve, others have reported significant temporal variability in speleothem DCF associated with changes in cave recharge. To further assess the potential hydrological control on speleothem radiocarbon variability, we constructed a new high-resolution DCF record from a speleothem from Flores, Indonesia for two different time periods, the Younger Dryas (YD) chronozone and the Last Millennium. A total of thirty-four 14C analyses (twenty for the YD and fourteen for the Last Millennium) were conducted on pieces of calcite extracted from stalagmite LR06-B1, which was well-dated by ~90 U-Th ages. To better characterize the paleoclimate and environmental changes, high-resolution stable-isotope (δ18O, δ13C) and trace-element (Mg/Ca, Sr/Ca) measurements were also conducted along the same sections of stalagmite. Broad comparison of the DCF record with the hydrologically-controlled proxy data suggests that increases in rainfall were matched by DCF increases. In line with a previous interpretation of DCF variability for the same specimen, but during the time interval 2.4-2.8 cal kyr BP and the post-bomb period, we interpret the DCF during the YD and the Last Millennium to have been primarily controlled by limestone dissolution associated with changes in open- versus closed-system conditions, rather than other potential factors such as kinetic fractionation and/or variations in the age-spectrum of soil organic matter above the cave. American Geophysical Union, Fall Meeting 2015
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    Indo-Pacific hydroclimate over the past millennium and links with global climate variability
    (American Geophysical Union, 2016-01-01) Griffiths, ML; Drysdale, RN; Kimbrough, AK; Hua, Q; Johnson, KR; Gagan, MK; Cole, JE; Cook, BI; Zhao, JX; Hellstrom, JC; Hantoro, WS
    The El Niño-Southern Oscillation (ENSO) and Interdecadal Pacific Oscillation (IPO) are the dominant modes of hydroclimate variability in the tropical Pacific and have far-reaching impacts on Earth’s climate. Experiments combining instrumental records with climate-model simulations have highlighted the dominant role of the Pacific Walker circulation in shaping recent trends in global temperatures (Kosaka and Xie, 2013, 2016). However, the paucity of high-resolution terrestrial paleoclimate records of deep atmospheric convection over the Indo-Pacific Warm Pool (IPWP) precludes a comprehensive assessment as to role of the tropical Pacific in modulating radiative-forced shifts in global temperature on multidecadal to centennial timescales. Here we present a suite of new high-resolution oxygen-isotope records from Indo-Pacific speleothems, which, based on modern rainfall and cave drip-water monitoring studies, along with trace element (Mg/Ca, Sr/Ca) analyses, are interpreted to reflect changes in Australasian monsoon variability during the Common Era (C.E.). Our results reveal a protracted decline in southern Indonesian monsoon rainfall between ~1000-1400 C.E. but stronger between ~1500-1900 C.E. These centennial-scale patterns over southern Indonesia are consistent with other proxy records from the region but anti-phased with records from India and China, supporting the paradigm that Northern Hemisphere cooling increased the interhemispheric thermal gradient, displacing the Australasian ITCZ southward. However, our findings are also compatible with a recent synthesis of paleohydrologic records for the Australasian monsoon region, which, collectively, suggest that rather than moving southward during the LIA, the latitudinal range of monsoon-ITCZ migration probably contracted equatorward (Yan et al., 2015). This proposed LIA ITCZ contraction likely occurred in parallel with a strengthening of the Walker circulation (as indicated through comparison with our hydroclimate records from the central-eastern equatorial Pacific Ocean and western Indian Ocean, and eastern Australia), and thus, the tropical Pacific may have played a critical role in amplifying the radiative-forced global cooling already underway. © 2016. American Geophysical Union
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    Rainfall variability and temporal changes in the dead carbon fraction in an Indonesian speleothem
    (Australasian Quaternary Association Inc., 2016-01-01) Hua, Q; Griffiths, ML; Drysdale, RN; Bajo, P; Jenkins, D; Hellstrom, JC; Johnson, KR; Gagan, MK; Zhao, JX
    The number of speleothem-based paleoclimate records has increased significantly in recent years. To assess the potential hydrological control on speleothem radiocarbon variability, we constructed a high-resolution dead carbon fraction (DCF) record from a speleothem from Flores, Indonesia for two different periods, the Younger Dryas (YD) chronozone and the Last Millennium. A total of thirty-four 14C analyses were conducted on calcite extracted from U-Th dated stalagmite LR06-B1. To better characterise the paleoclimate and environmental changes, highresolution stable-isotope (δ18O, δ13C) and trace-element (Mg/Ca, Sr/Ca) measurements were also conducted along the same stalagmite sections. Broad comparison of the DCF record with the hydrologically-controlled proxy data suggests that rainfall increases were matched by DCF increases. In line with a previous interpretation of DCF variability for the same specimen, but during the interval 2.4-2.8 ka and the post-bomb period, we interpret the DCF during the YD and the Last Millennium to have been primarily controlled by limestone dissolution associated with changes in open- versus closed-system conditions, rather than other potential factors such as kinetic fractionation and/or variations in the age-spectrum of soil organic matter above the cave. It then follows that more abundant monsoon rainfall in Flores resulted in the soil-karst system being in a more closed state, which inhibited carbon isotope exchange between the karst-water dissolved inorganic carbon and soil-gas CO2, and ultimately led to a greater contribution of dead-carbon from the bedrock. Our results indicate that DCF in tropical speleothems can be used as a proxy of past rainfall and consequently monsoon variability.