Browsing by Author "Mankey, GJ"

Now showing 1 - 11 of 11
  • No Thumbnail Available
    Item
    Antiferromagnetism in a Fe50Pt40Rh10 thin film investigated using neutron diffraction
    (American Physical Society, 2008-11) Lott, D; Fenske, J; Schreyer, A; Mani, P; Mankey, GJ; Klose, F; Schmidt, W; Schmalzl, K; Tartakovskaya, EV
    The temperature-dependent magnetic structure of a 200 nm thick single-crystalline film of Fe50Pt40Rh10 was studied by unpolarized and polarized neutron diffractions. By applying structure factor calculations, a detailed model of the magnetic unit cell was developed. In contrast to former studies on bulk samples, our experimental results show that the film remains in an antiferromagnetic state throughout the temperature range of 10–450 K. Remarkably, it can be demonstrated that the antiferromagnetic structure undergoes a smooth transition from a dominant out-of-plane order with the magnetic moments orientated in-plane to an in-plane order with the magnetic moments orientated perpendicular to the film plane. Theoretically this can be explained by the existence of two competing anisotropy contributions with different temperature dependencies. © 2008, American Physical Society
  • No Thumbnail Available
    Item
    Artificially modulated chemical order in thin films: a different approach to create ferro/antiferromagnetic interfaces
    (American Physical Society, 2010-10-06) Saerbeck, T; Klose, F; Lott, D; Mankey, GJ; Lu, Z; LeClair, PR; Schmidt, W; Stampfl, APJ; Danilkin, SA; Yethiraj, M; Schreyer, A
    We report on a unique magnetic exchange interaction in a thin film of FePt3, comprising an artificially created ferromagnetic (FM)/antiferromagnetic (AFM) modulation, but homogeneous chemical composition and epitaxy throughout the film. The chemical order, on the other hand, is modulated resulting in the formation of alternating FM/AFM layers. To determine the existence and form of the magnetic structure within the monostoichiometric thin film, we use a unique combination of polarized neutron reflectometry, x-ray/neutron diffraction, and conventional magnetometry. This artificial stratified AFM/FM FePt3 exhibits a high magnetic exchange bias thus opening up possibilities to study such magnetic phenomena in a perfectly lattice-matched system. © 2010, American Physical Society
  • No Thumbnail Available
    Item
    Chemical-order-induced magnetic exchange bias in epitaxial FePt3 films
    (American Physical Society, 2008-04-11) Lott, D; Klose, F; Ambaye, H; Mankey, GJ; Mani, P; Wolff, M; Schreyer, A; Christen, HM; Sales, BC
    We show that magnetic exchange bias can be induced by means of chemical ordering. The effect was observed on epitaxial thin film layers of FePt3, a material which has the remarkable property that, depending on the degree of chemical order, a ferromagnetic and an antiferromagnetic magnetic state can coexist at the same temperature. We demonstrate that the observed exchange bias originates at the interfaces between these two different magnetic phases of FePt3. © 2008, American Physical Society
  • Thumbnail Image
    Item
    Depth control of ferromagnetism in FePt3 films by ion-irradiation
    (International Conference on Neutron Scattering, 2017-07-12) Causer, GL; Cortie, DL; Zhu, HL; Ionescu, M; Mankey, GJ; Klose, F
    The roadmap which outlines storage technology of magnetic hard disk drives predicts storage densities above 5 Tb/in2 to be realised by isolated, individually addressable ferromagnetic (FM) bits of <10 nm in lateral dimension. In principle, artificially patterned structures of this type can be manufactured by x-ray, ion-and electron-beam lithography. However, there may be alternative solutions for obtaining these regular, nanoscale patterns of isolated FM dots. Our proposal is to locally transform a non-magnetic layer into a pattern of geometrically defined FM islands. Such a phase transition could be initiated by locally changing some physical parameter of the layer, such as its strain state or chemical composition leading to ferromagnetism. Here, we present a chemical order (paramagnetic) to chemical disorder (FM) phase transition stimulated by He+ irradiation of a FePt3 thin film. This talk will present preliminary work focussing on depth profiling the ion-beam induced FM order. By controlling the energy (15 keV) and fluence (2x1016 ions/cm2) of the ion-beam, we show ferromagnetism can be locally induced into the upper-half volume of the initially chemically well-ordered 280 nm FePt3 film. Polarised neutron reflectometry was used to investigate the depth dependence of the layer averaged ion-beam induced FM moment within the thin film. Data analysis of the Kiessig fringes observed in the reflectivity post-irradiation suggest the FM / nonmagnetic interface is atomically sharp. The resulting bilayer structure was found to be homogenous in chemical composition but heterogeneous in both chemical and magnetic orders.
  • No Thumbnail Available
    Item
    Depth-profiling magnetic interfaces formed intrinsically in FePt3 by ion-beams
    (American Physical Society, 2018-03-07) Causer, GL; Cortie, DL; Zhu, HL; Ionescu, M; Mankey, GJ; Wang, XL; Klose, F
    Using ion-beams to locally modify material properties is rapidly gaining momentum as a technique of choice for the fabrication of magnetic nano-elements because the method provides the capability to nano-engineer in 3D, which is important for many future spintronic technologies. The precise definition of the resulting element shape is crucial for device functionality. In this work, the intrinsic sharpness of a magnetic interface formed by nano-machining FePt3 films using He+ irradiation is investigated. Through careful selection of the irradiating ion’s energy and fluence, ferromagnetism is locally induced into a fractional volume of a paramagnetic (PM) FePt3 film by modifying the chemical order parameter. Using a combination of magnetometry, transmission electron microscopy and polarised neutron reflectometry it is demonstrated that the interface over which the PM to ferromagnetic modulation occurs is confined to a few atomic monolayers only. Using density functional theory, the mechanism for the ion-beam induced magnetic transition is elucidated and shown to be caused by an intermixing of Fe and Pt atoms in anti-site defects above a threshold density.
  • No Thumbnail Available
    Item
    High magnetization FeCo/Pd multilayers
    (American Vacuum Society, 2008-07) Walock, MJ; Ambaye, H; Chshiev, M; Klose, F; Butler, WH; Mankey, GJ
    We have fabricated multilayer samples with varying superlattice periodicity and interlayer thicknesses to determine the nature of the enhanced moment in this intriguing thin film system. Magnetic characterization experiments show an enhanced magnetic moment in the multilayers as compared to a single layer film containing the same amount of FeCo. However, since the magnetization is defined as the magnetic moment divided by the sample volume, the sample exhibits an overall reduction in the magnetization when the volume of the Pd layers is also taken into account. Our experimental findings are also supported by theoretical calculations which identify the origin of the increased magnetic moment in the multilayer system. Polarized neutron reflectivity experiments will be used to determine the lateral distribution of the magnetization in a number of superlattice samples. © 2008, American Vacuum Society
  • Thumbnail Image
    Item
    Magnetic interface phenomena in nano-architectures and their applications
    (Australian Institute of Nuclear Science and Engineering (AINSE), 2018-11-19) Causer, GL; Cortie, DL; Zhu, HL; Kostylev, M; Ionescu, M; Mankey, GJ; Wang, XL; Klose, F
    Interfaces between heterostructure components in nanoscale films play important roles in communicating low-dimensional phenomena and act as anchor points for the direct control and tunability of device performance. In this talk I will give an overview of our group’s recent investigations into the occurrence of magnetic interface phenomena in low-dimensional thin-film systems which have conceivable utility in future condensed-matter technologies. First, the magnetic interface quality of an FePt3 nano-magnet formed via ion-induced chemical disorder will be analysed [1]. Here, neutron and electron measurements used in combination with density functional theory calculations reveal a rather counterintuitive result which could prove beneficial towards the development of ultra-high density magnetic recording devices. In a second study, the layer-averaged static magnetisation and macroscopic magneto-dynamic behaviours of a Co/Pd bilayer during hydrogen-gas cycling are analysed. To perform this characterisation, we first had to develop and commission an original sample environment which innovatively combines polarised neutron reflectometry and microwave spectroscopy [2]. The Co/Pd interface is found to feature tailorable magnetic surface anisotropy in the presence of hydrogen gas – the mechanism of which could act as a safety switch in next-generation vehicles powered by hydrogen.
  • Thumbnail Image
    Item
    A new approach to the creation of magnetically modulated structures
    (Australian Institute of Physics, 2010-02-03) Saerbeck, T; Klose, F; Lott, D; Mankey, GJ; Lu, Z; LeClair, PR; Stampfl, APJ; Danilkin, SA; Yethiraj, M; Schreyer, A
    The plethora of structural and magnetic properties observed in many transition metal alloys has attracted a great deal of interest in both the pure and applied sciences [1]. One key attribute of these alloys is that their electronic and magnetic properties are extremely sensitive to not only stoichiometry but order as well. In this paper we report on a new approach of creating a magnetically modulated structure, without changing composition or lattice structure, namely by artificially controlling the degree of chemical order in the material. The compound FePt3, as it is well known from bulk crystals, has the extraordinary property to evolve ferromagnetic (FM) or antiferromagnetic (AFM) phases determined by the degree of chemical ordering [2]. We succeeded in preparing epitaxial FePt3 superlattices of homogeneous composition consisting of an artificially modulated ferro/antiferromagnetic layering sequence simply by alternating the growth temperature. A direct effect of such an exotic FM/AFM interface is the observation of a high exchange bias upon field cooling through the Nèel temperature. In order to quantify the degree of antiferromagnetic ordering, high angle neutron diffraction has been performed using the triple axis spectrometer IN12 (Institute Laue Langevin, Grenoble) and TAIPAN (Australian Nuclear Science and Technology Organisation). Similar to chemically ordered bulk FePt3 the superlattice exhibits the onset of a (½ ½ 0) AFM Bragg peak below a temperature of TN=140 K (Bulk TN=160 K [2]). Using the polarized neutron reflectometry technique at the German research facility GKSS, Geesthacht, a detailed layer resolved magnetic characterization of the superlattice was carried out.
  • No Thumbnail Available
    Item
    Polarized neutron reflectometry of epitaxial Fe[0.25 + x] Pt[0.75 – x] layers.
    (Institute of Electrical and Electronics Engineers (IEEE), 2018-04-27) Mankey, GJ; Causer, GL; Cortie, DL; Wang, X; Zhu, H; Lonescu, M; Klose, F
    Epitaxial Fe[0.25 + x]Pt[0.75 - x] layers can be either antiferromagnetic (AF) or ferromagnetic (FM) depending on the degree of chemical ordering controlled by the deposition temperature. Our neutron diffraction studies were the first to study AF phase transitions in these thin films [1] and we have also shown using PNR that a mixed AF-FM film is exchange biased with itself [2]. In AF-FM exchange-biased superlattices with a modulated chemical order parameter, PNR shows the magnetization can be modulated through the film thickness with no composition modulations [3]. Our recent results reveal that He+ ion bombardment and annealing can be applied toward controlling magnetic phases in epitaxial Fe [0.25] Pt [0.75] layers [4]. © Copyright 2024 IEEE - All rights reserved, including rights for text and data mining and training of artificial intelligence and similar technologies.
  • No Thumbnail Available
    Item
    Structural and magnetic properties of epitaxial Fe25Pt75
    (American Vacuum Society, 2009-07) Lu, Z; Walock, MJ; LeClair, PR; Mankey, GJ; Mani, P; Lott, D; Klose, F; Ambaye, H; Lauter, V; Wolff, M; Schreyer, A; Christen, HM; Sales, BC
    Epitaxial films of Fe25Pt75 have a number of different magnetic phases as a function of temperature and chemical order. For example, chemically ordered epitaxial films have two distinct antiferromagnetic phases at temperatures below similar to 160 K and exhibit paramagnetism above that temperature. In sharp contrast, chemically disordered epitaxial films are ferromagnetic with a Curie temperature that is greater than 400 K. It is demonstrated that by varying the substrate temperature during growth, epitaxial films with varying degrees of chemical order can be produced and it is possible to produce an alloy with the same composition throughout the film with a modified magnetic structure. The authors used polarized neutron reflectivity to gauge the magnetism of a Fe25Pt75 sample produced with a periodic variation in the growth temperature and showed that the sample exhibits a reduced Curie temperature of approximately 300 K as compared to bulk Fe25Pt75. © 2009, American Vacuum Society
  • No Thumbnail Available
    Item
    Tailoring exchange bias through chemical order in epitaxial FePt3 films
    (AIP Publishing, 2013-01-01) Saerbeck, T; Zhu, HL; Lott, D; Lee, H; LeClair, PR; Mankey, GJ; Stampfl, APJ; Klose, F
    Intentional introduction of chemical disorder into mono-stoichiometric epitaxial FePt3 films allows to create a ferro-/antiferromagnetic two-phase system, which shows a pronounced and controllable exchange bias effect. In contrast to conventional exchange bias systems, granular magnetic interfaces are created within the same crystallographic structure by local variation of chemical order. The amount of the exchange bias can be controlled by the relative amount and size of ferromagnetic and antiferromagnetic volume fractions and the interface between them. The tailoring of the magnetic composition alone, without affecting the chemical and structural compositions, opens the way to study granular magnetic exchange bias concepts separated from structural artifacts. © 2013, American Institute of Physics.