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Please use this identifier to cite or link to this item: http://apo.ansto.gov.au/dspace/handle/10238/4897

Title: In-Situ Study of Catalytic Processes: Neutron Diffraction of a Methanol Synthesis Catalyst at Industrially Relevant Pressure
Authors: Kandemir, T
Girgsdies, F
Hansen, TC
Liss, KD
Kasatkin, I
Kunkes, EL
Wowsnick, G
Jacobsen, N
Schlögl, R
Behrens, M
Keywords: COPPER
IRON
SCATTERING
HYDROGEN
NEUTRON DIFFRACTION
CATALYSTS
Issue Date: 1-Jan-2013
Publisher: Wiley-V C H Verlag GMBH
Citation: Kandemir, T., Girgsdies, F., Hansen, T. C., Liss, K.-D., Kasatkin, I., Kunkes, E. L., Wowsnick, G., Jacobsen, N., Schlögl, R., & Behrens, M. (2013). In-Situ Study of Catalytic Processes: Neutron Diffraction of a Methanol Synthesis Catalyst at Industrially Relevant Pressure. Angewandte Chemie International Edition, 52 (19), 5166-5170.
Abstract: An industrial methanol synthesis catalyst operating at high pressure was studied by in situ neutron diffraction. The peculiar microstructure of Cu/ZnO/Al2O3 nanocatalysts was found to be stable under reaction conditions. Stacking fault annealing and brass formation was only observed at temperatures higher than used in the methanol synthesis process, providing support for active role of defects in this catalyst system. © 2013, Wiley-VCH Verlag.
URI: http://dx.doi.org/10.1002/anie.201209539
http://apo.ansto.gov.au/dspace/handle/10238/4897
ISSN: 1433-7851
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