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Title: In-Situ Study of Catalytic Processes: Neutron Diffraction of a Methanol Synthesis Catalyst at Industrially Relevant Pressure
Authors: Kandemir, T
Girgsdies, F
Hansen, TC
Liss, KD
Kasatkin, I
Kunkes, EL
Wowsnick, G
Jacobsen, N
Schlögl, R
Behrens, M
Keywords: Copper
Neutron diffraction
Issue Date: 1-Jan-2013
Publisher: Wiley-V C H Verlag GMBH
Citation: Kandemir, T., Girgsdies, F., Hansen, T. C., Liss, K.-D., Kasatkin, I., Kunkes, E. L., Wowsnick, G., Jacobsen, N., Schlögl, R., & Behrens, M. (2013). In-situ study of catalytic processes: neutron diffraction of a methanol synthesis catalyst at industrially relevant pressure. Angewandte Chemie International Edition, 52 (19), 5166-5170. doi:10.1002/anie.201209539
Abstract: An industrial methanol synthesis catalyst operating at high pressure was studied by in situ neutron diffraction. The peculiar microstructure of Cu/ZnO/Al2O3 nanocatalysts was found to be stable under reaction conditions. Stacking fault annealing and brass formation was only observed at temperatures higher than used in the methanol synthesis process, providing support for active role of defects in this catalyst system. © 2013, Wiley-VCH Verlag.
Gov't Doc #: 5113
ISSN: 1433-7851
Appears in Collections:Journal Articles

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