Browsing by Author "Sato, TJ"
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- ItemAntiferromagnetic order of ferromagnetically coupled dimers in the double pyrovanadate CaCoV2O7(Cornell University, 2021-08-02) Murasaki, R; Nawa, K; Okuyama, D; Avdeev, M; Sato, TJMagnetic properties of the pyrovanadate CaCoV2O7 have been studied by means of the bulk magnetization and neutron powder diffraction measurements. Magnetic susceptibility in the paramagnetic phase shows Curie-Weiss behavior with negative Weiss temperature ≃ −22.5 K, indicating dominant antiferromagnetic interactions. At TN = 3.44 K, CaCoV2O7 shows antiferromagnetic order, accompanied by a weak net ferromagnetic moment of ∼ 0.05 μB/Co2+. Neutron powder diffraction confirms the formation of antiferromagnetic order below TN. It was further confirmed from the magnetic structure determination that the two Co2+ ions in the adjacent edge-sharing octahedra have almost parallel (ferromagnetic) spin arrangement, indicative of a formation of a ferromagnetic spin dimer. The antiferromagnetic order is, in turn, stabilized by sizable inter-dimer antiferromagnetic interactions.
- ItemBlock magnetism coupled with local distortion in the iron-based spin-ladder compound BaFe 2 Se 3(American Physical Society, 2012-02-22) Nambu, Y; Ohgushi, K; Suzuki, S; Du, F; Avdeev, M; Uwatoko, Y; Munakata, K; Fukazawa, H; Chi, S; Ueda, Y; Sato, TJMagnetism in the insulating BaFe2Se3 was examined through susceptibility, specific heat, resistivity, and neutron diffraction measurements. After formation of a short-range magnetic correlation, a long-range ordering was observed below TN∼255 K. The transition is obscured by bulk properties. Magnetic moments (∥a) are arranged to form a Fe4 ferromagnetic unit, and each Fe4 stacks antiferromagnetically. This block magnetism is of the third type among magnetic structures of ferrous materials. The magnetic ordering drives unusually large distortion via magnetoelastic coupling. ©2012 American Physical Society
- ItemControlling the stoichiometry of the triangular lattice antiferromagnet Li1+xZn2-yMo3O8(The Physical Society of Japan, 2017-09-12) Sandvik, KE; Nawa, K; Okuyama, D; Reim, J; Avdeev, M; Matsuda, M; Sato, TJAn intriguing topic in condensed matter physics is exploring exotic ground states in frustrated quantum systems, such astriangular-or kagome-lattice antiferromagnets. In these systems competing interactions destabilize conventional magnetic order and lead to interesting nonmagnetic states, exemplified by the quantum spin liquid or resonating valence bond state.The compound LiZn2Mo3O8(LZMO) is an antiferromagnet with magnetic Mo3O13 clusters forming triangular layers well separated from each other. It is proposed to realize a condensed valence bond state [1]. For the stoichiometric composition, these clusters have an unpaired electron (spin 1/2) and hence the system may be an ideal playground for exploring exotic ground states in quantum triangular antiferromagnet. However, chemical disorder atLi/Zn cites in LZMO easily leads to off-stoichiometry that introduces unoccupied S= 1/2 sites in the triangular lattice.Partial control of the Zn composition has been achieved by earlier efforts involving electrochemical technique[2], however,full stoichiometry control has not been achieved as far as we know. Since the stoichiometry is the key to explore intrinsic physics in the quantum S= 1/2 triangular antiferromagnet, we undertook a thorough investigation on the relation between initial and final chemical composition for the LZMO system. Several LZMO compounds were prepared using solid-state reaction technique [1] with widely varied starting composition. After the reactions, the samples were washed by hydrochloric acid to remove excess ZnO. The composition of the obtained compounds was determined as Li1+xZn2-yMo3O8from ICP mass spectroscopy (ArcosEOP, Spectro), X-ray diffraction (Rigaku) and neutron powder diffraction (Echidna, ANSTO). Composition dependence on the magnetism was investigated using the magnetic property measurement system (MPMS-XL, Quantum Design). © 2017 The Physical Society of Japan
- ItemControlling the stoichiometry of the triangular lattice antiferromagnet Li1+xZn2−yMo3O8(Elsevier, 2019-01-03) Sandvik, KE; Okuyama, D; Nawa, K; Avdeev, M; Sato, TJThe control of the stoichiometry of Li1+xZn2−yMo3O8 was achieved by the solid-state-reaction. We found that the best sample that has the chemical composition Li0.95(4)Zn1.92(8)Mo3O8 was obtained from the starting nominal composition with Li : Zn : Mo : O=(1+w) : (2.8−w) : 3 : 8.6 with w=−0.1, indicating that the stoichiometry is greatly improved compared to those in the earlier reports. For larger w detailed structural analysis indicates that the mixed sites of Li and Zn are preferentially occupied by Li atoms, as well as the fraction of the non-magnetic secondary phase Zn2Mo3O8 decreases. Magnetic susceptibility of the improved stoichiometry powder samples shows a broad hump in the temperature range of 100
- ItemCrystal structure and magnetic properties of the breathing kagome ising antiferromagnet Yb3Ni11Ge4.63(The Physical Society of Japan, 2020-07-31) Takahashi, M; Nawa, K; Okuyama, D; Nojiri, H; Frontzek, MD; Avdeev, M; Yoshida, M; Ueta, D; Yoshizawa, H; Sato, TJWe have investigated magnetic properties of the rare-earth based intermetallic compound Yb3Ni11Ge4.63 (YNG), where Yb3+ ions form a breathing-kagome lattice. Single-site 4f electron wavefunctions of the ground-state doublet are deduced from magnetization and heat capacity measurements. The Weiss temperatures are quite anisotropic as Θa = −0.01(2) K (H ∥ a) and Θc = −0.67(2) K (H ∥ c), indicating Ising-like spin–spin interactions dominating in this compound. Low-temperature neutron diffraction confirms absence of magnetic Bragg peaks down to 0.05 K, whereas enhancement of broad peaks below 0.8 K was observed, a signature of short-range spin correlations. Competing interactions on the breathing-kagome lattice would suppress a magnetic long-range order in YNG. ©2020 The Physical Society of Japan
- ItemDegenerate ground state in the classical pyrochlore antiferromagnet Na3Mn(CO3)2Cl(American Physical Society, 2018-10-18) Nawa, K; Okuyama, D; Avdeev, M; Nojiri, H; Yoshida, M; Ueta, D; Yoshizawa, H; Sato, TJIn an ideal classical pyrochlore antiferromagnet without perturbations, an infinite degeneracy in a ground state leads to the absence of magnetic order and a spin-glass transition. Here we present Na3Mn(CO3)2Cl as a new candidate compound where classical spins are coupled antiferromagnetically on the pyrochlore lattice and report its structural and magnetic properties. The temperature dependences of the magnetic susceptibility and heat capacity and the magnetization curve are consistent with those of an S=5/2 pyrochlore lattice antiferromagnet with nearest-neighbor interactions of 2 K. Neither an apparent signature of a spin-glass transition nor magnetic order is detected in magnetization and heat capacity measurements or powder neutron diffraction experiments. On the other hand, antiferromagnetic short-range order of the nearest neighbors is evidenced by the Q dependence of the diffuse scattering which develops around 0.85Å−1. A high degeneracy near the ground state in Na3Mn(CO3)2Cl is supported by the magnetic entropy, estimated as almost 4JK−2mol−1 at 0.5 K. ©2018 American Physical Society
- ItemErratum: Magnetic structure and dzyaloshinskii-moriya interaction in the S=1/2 helical-honeycomb antiferromagnet α−Cu2V2O7 [Phys. Rev. B 92, 024423 (2015)](American Physical Society, 2017-03-10) Gitgeatpong, G; Zhao, Y; Avdeev, M; Piltz, RO; Sato, TJ; Matan, KNo abstract available. See the original item at: https://apo.ansto.gov.au/dspace/handle/10238/10250
- ItemExperimental observation of long-range magnetic order in icosahedral quasicrystals(American Chemical Society, 2021-11-17) Tamura, R; Ishikawa, A; Suzuki, S; Kotajima, T; Tanaka, Y; Seki, T; Shibata, N; Yamada, T; Fujii, T; Wang, CW; Avdeev, M; Nawa, K; Okuyama, D; Sato, TJQuasicrystals (QCs), first discovered in 1984, generally do not exhibit long-range magnetic order. Here, we report on long-range magnetic order in the real icosahedral quasicrystals (i QCs) Au–Ga–Gd and Au–Ga–Tb. The Au65Ga20Gd15i QC exhibits a ferromagnetic transition at TC = 23 K, manifested as a sharp anomaly in both magnetic susceptibility and specific heat measurements, along with an appearance of magnetic Bragg peak below TC. This is the first observation of long-range magnetic order in a real quasicrystal, in contrast to the spin-glass-like behaviors observed for the other magnetic quasicrystals found to date. Moreover, when Gd is replaced by Tb, i.e., for the Au65Ga20Tb15i QC, a ferromagnetic behavior is still retained with TC = 16 K. Although the sharp anomaly in the specific heat observed for the Au65Ga20Gd15i QC becomes broadened upon Tb substitution, neutron diffraction experiments clearly show marked development of magnetic Bragg peaks just below TC, indicating long-range magnetic order for the Au65Ga20Tb15i QC also. Our findings can contribute to the further investigation of exotic magnetic orders formed on real quasiperiodic lattices with unprecedented highest global symmetry, i.e., icosahedral symmetry. © 2021 The Authors - CC BY. Published by American Chemical Society
- ItemFrustrated magnetism in the J1−J2 honeycomb lattice compounds MgMnO3 and ZnMnO3 synthesized via a metathesis reaction(American Physical Society, 2019-12-17) Haraguchi, Y; Nawa, K; Michioka, C; Ueda, J; Matsuo, A; Kindo, K; Avdeev, M; Sato, TJ; Yoshimura, KWe investigated the magnetic properties of the ilmenite-type manganates MgMnO3 and ZnMnO3, both of which are composed of a honeycomb lattice of magnetic Mn4+ ions. Both compounds show antiferromagnetic order with weak ferromagnetic moments. In particular, MgMnO3 exhibits a magnetization “reversal” behavior which can be described by the N-type ferrimagnetism in the Néel's classification. The relationship between the magnetic properties and the crystal and magnetic structures probed by the neutron diffraction experiments indicates that the two honeycomb lattice magnets have different J1−J2 parameter sets, placing them in the distinct regions in the phase diagram; both nearest neighbor (NN) and next nearest neighbor (NNN) exchange interactions are antiferromagnetic in MgMnO3, while NN and NNN interactions become ferromagnetic and antiferromagnet, respectively, in ZnMnO3. ©2019 American Physical Society
- ItemHelical magnetic structure in cubic chiral crystal Pr5Ru3Al2(International Union of Crystallography, 2017-01-01) Okuyama, D; Makino, K; Avdeev, M; Ohishi, K; Yamauchi, K; Oguchi, T; Sato, TJHelical magnetic structure has recently attracted intrests because of the discovery of novel topological spin textures, forexample magnetic skyrmions and chiral magnetic soliton lattices. For such spin textures, a finite antisymmetricDzyaloshinsky–Moriya-type (cross product) interaction is crucial, activated in noncentrosymmetric crystals. Suchantisymmetric interactions have been studied mainly in 3d magnets. For example, in B20 compound (Mn,Fe,Co)Ge, theantisymmetric interaction is well investigated by the theoretical first principle calculation and found that the observed signinversion of the helicity of the helical magnetic structure by the magnetic ion substitution is quantitatively explained [1]. Incontrast, there are few studies investigating the antisymmetric interaction in 4f rare-earth based noncentrosymmetricmaterials. Murashova et al. reported the rare-earth based chiral compounds Re5Ru3Al2 with the space group I213 (Re = La,Pr) [2]. Nonetheless, their low temperature magnetism was largely unexplored. Powder Pr5Ru3Al2 was synthesized by the arc melting and high-frequency induction heating methods. The powder sampleswere annealed using muffle furnace and the high quality powder sample and single crystal were grown. In the magnetizationmeasurement using obtained Pr5Ru3Al2, the temperature dependence of the magnetic susceptibility is fitted by Curie-Weisslaw and the obtained Curie constant is close to the value for a free Pr3+ ion. At 4K, the antiferromagnetic transition isobserved [3]. To clarify the magnetic structure of Pr5Ru3Al2, we performed powder neutron diffraction using ECHIDNA inANSTO and single crystal small angle neutron scattering (SANS) using TAIKAN in J-PARC. The powder diffraction pattern at10 K is explained by the nuclear scattering of Pr5Ru3Al2. At 3 K, additional incommensurate magnetic peaks with thepropagation vector (q q q): q ~ 0.066 [r. l. u.] are observed. More noteworthy are the integrated intensities of theequivalent magnetic reflections around the nuclear 1 1 0 are not the same value. To explain the difference of the intensitiesbetween equivalent reflections, it is reasonable to conclude that the helical magnetic ordering takes place and the sign of itshelicity is determined by the sign of the crystal chirality. The magnetic structure determined by the magnetic representationand Rietveld analyses is shown in Fig. 1 (a). The composite magnetic structure obtained by adding the magnetic moments ofPr1, Pr2, Pr3, and Pr4 layers is the typical helical, as shown in Fig. 1 (b). In the SANS experiment using single crystalPr5Ru3Al2, the (q q q)-type magnetic reflection is also observed below 3.3 K. The band structure near Fermi energy iscalculated by the first principle calculation to determine the conduction band mediating RKKY interaction. From theseexperimental and theoretical results, the origin of the helical magnetic structure in Pr5Ru3Al2 will be discussed. © International Union of Crystallography
- ItemIncommensurate magnetic structure in the cubic noncentrosymmetric ternary compound Pr5Ru3Al2(The Physical Society of Japan, 2016-06-08) Makino, K; Okuyama, D; Avdeev, M; Sato, TJMagnetic susceptibility and neutron powder diffraction experiments have been performed on the noncentrosymmetric ternary compound Pr5Ru3Al2. The previously reported ferromagnetic transition at 24 K was not detected in our improved-quality samples. Instead, magnetic ordering was observed in the DC magnetic susceptibility at Tc≃3.8 K. The neutron powder diffraction experiment further indicates that an incommensurate magnetic structure is established below Tc with the magnetic modulation vector q≃(0.066,0.066,0.066) ©2016 The Physical Society of Japan
- ItemMagnetic and transport properties of AFe_2Se_3 (A= Ba and Cs)(The Physical Society of Japan, 2012-03-05) Du, F; Ohgushi, K; Sasaki, R; Matsubayashi, K; Uwatoko, Y; Kawakami, T; Nambu, Y; Avdeev, M; Sato, TJ; Ueda, YThe orthorhombic AFe2Se3 (A=Ba and Cs) have attracted much attention due to the possibility of superconducivity AFe2Se3 The crystal structure of 14Fe2Se3 can be described as double chains of [Fe2Se3】formed by the edge sharing FeSe4 tetrahedra. We synthesize AFezSe3 single crystalline samples by the self flux method firstly, then studies the magnetic and transport properties under ambient and high pressure. BaFe2Se3 shows a semiconducting behavior. With increasing pressure 8 GPa, the charge gap of BaFe2Se3 gradually decreases; however, the ground state is still insulating at 8 GPa. Interestingly, CBFe2Se3 also shows a Semiconducting behavior although the formally mixed valence state of Fe ions. Mossbauer spectra of CsFe2Se3 indicate that electronic state of Fe ions is unique, ruling out the possibility of charge ordering. In addition, a magnetic transition at 170K is suggested from the hyperfine filed splitting in the Mossbauer spectra and neutron diffraction analysis．
- ItemMagnetic properties and magnetic structure of the frustrated quasi-one-dimensional antiferromagnet SrCuTe2O6(American Physical Society, 2020-10-07) Saeaun, P; Zhao, Y; Piyawongwatthana, P; Sato, TJ; Chou, FC; Avdeev, M; Gitgeatpong, G; Matan, KMagnetization measurements on single-crystal cubic SrCuTe2O6 with an applied magnetic field along three inequivalent high symmetry directions [100], [110], and [111] reveal weak magnetic anisotropy. The fits of the magnetic susceptibility to the result from a quantum Monte Carlo simulation on the Heisenberg spin-chain model, where the chain is formed via the dominant third-nearest-neighbor exchange interaction J3, yield the intrachain interaction (J3/kB) between 50.12(7) K for the applied field along [110] and 52.5(2) K along [100] with about the same g factor of 2.2. Single-crystal neutron diffraction unveils the transition to the magnetic ordered state as evidenced by the onset of the magnetic Bragg intensity at TN1=5.25(9)K with no anomaly of the second transition at TN2 reported previously. Based on irreducible representation theory and magnetic space group analysis of powder and single-crystal neutron diffraction data, the magnetic structure in the Shubnikov space group P4132, where the Cu2+S=1/2 spins antiferromagnetically align in the direction perpendicular to the spin chain, is proposed. The measured ordered moment of 0.52(6)μB, which represents 48% reduction from the expected value of 1μB, suggests the remaining influence of frustration resulting from the J1 and J2 bonds. ©2020 American Physical Society
- ItemMagnetic properties of the S = 1/2 antiferromagnetic spin-chain α - Cu2V2O7(American Physical Society, 2015-03-06) Gitgeatpong, G; Zhao, Y; Avdeev, M; Piltz, RO; Sato, TJ; Matan, KMagnetic properties of the S = 1 / 2 antiferromagnetic spin-chain, α - Cu2V2O7, have been studied using magnetization and neutron scattering measurements on powder and single-crystal samples. Magnetic susceptibility reveals a Curie-Weiss temperature of Θ = -73.2(9) K with a magnetic phase transition at TN = 33 K while the Bonner-Fisher fit to the magnetic susceptibility for T >TN with magnetic field perpendicular to the crystallographic a - axis yields the intra-chain coupling of |J|/k = 46.0(2) K. Small ferromagnetism below TN is due to spin-canting caused by Dzyaloshinskii-Moriya interactions. Analysis of the neutron diffraction data reveals that the Cu2+ spins are coupled antiferromagnetically along zigzag chains, which run alternately along [011] and [01-1] directions. The ordered moment of 0.925(3) μB is predominantly along the a - axis. Our recent inelastic neutron scattering, which reveals atypical magnetic excitations centered at commensurate wave vectors (0, +/-0.25, 0) around the magnetic zone center, will also be discussed. © 2021 American Physical Society
- ItemMagnetic structure and dzyaloshinskii-moriya interaction in the S=12 helical-honeycomb antiferromagnet α−Cu2V2O7(American Physical Society, 2015-07-23) Gitgeatpong, G; Zhao, Y; Avdeev, M; Piltz, RO; Sato, TJ; Matan, KMagnetic properties of the S=12 antiferromagnet α−Cu2V2O7 have been studied using magnetization, quantum Monte Carlo (QMC) simulations, and neutron diffraction. Magnetic susceptibility shows a broad peak at ∼50K followed by an abrupt increase indicative of a phase transition to a magnetically ordered state at TN=33.4(1) K. Above TN, a fit to the Curie-Weiss law gives a Curie-Weiss temperature of Θ=−73(1) K suggesting the dominant antiferromagnetic coupling. The result of the QMC calculations on the helical-honeycomb spin network with two antiferromagnetic exchange interactions J1 and J2 provides a better fit to the susceptibility than the previously proposed spin-chain model. Two sets of the coupling parameters J1:J2=1:0.45 with J1=5.79(1) meV and 0.65:1 with J2=6.31(1) meV yield equally good fits down to ∼TN. Below TN, weak ferromagnetism due to spin canting is observed. The canting is caused by the Dzyaloshinskii-Moriya interaction with an estimated bc-plane component |Dp|≃0.14J1. Neutron diffraction reveals that the S=12Cu2+ spins antiferromagnetically align in the Fd′d′2 magnetic space group. The ordered moment of 0.93(9) μB is predominantly along the crystallographic a axis. ©2015 American Physical Society
- ItemMagnetic structure of the S=1/2 quasi-two-dimensional square-lattice Heisenberg antiferromagnet Sr2CuTeO6(American Physical Society, 2016-02-26) Koga, T; Kurita, N; Avdeev, M; Danilkin, SA; Sato, TJ; Tanaka, HThe magnetic structure of the double perovskite compound Sr2CuTeO6 was determined from neutron powder diffraction data. This material is magnetically described as an S=1/2 quasi-two-dimensional square-lattice Heisenberg model with antiferromagnetic nearest-neighbor and next-nearest-neighbor interactions. Sr2CuTeO6 undergoes a magnetic phase transition at TN≃29 K. The spin structure below TN is Néel antiferromagnetic on the square lattice, which means that the nearest-neighbor interaction (J1) is stronger than the next-nearest-neighbor interaction (J2), in contrast to other isostructural compounds such as Ba2CuWO6 and Sr2CuWO6, for which |J1|<|J2| is realized. ©2016 American Physical Society
- ItemMagnetic structure study of the sawtooth chain antiferromagnet Fe2Se2O7(Springer Nature, 2021-12-15) Nawa, K; Avdeev, M; Berdonosov, P; Sobolev, A; Presniakov, I; Aslandukova, A; Kozlyakova, E; Vasiliev, AN; Shchetinin, I; Sato, TJA magnetic structure of the sawtooth-chain antiferromagnet Fe2Se2O7 was investigated by magnetization measurements, single crystalline and powder neutron diffraction experiments, and a further analysis on the Mössbauer spectra. These experiments revealed a nearly collinear antiferromagnetic structure with magnetic moments aligned along the b-axis, indicating dominant antiferromagnetic exchanges between Fe(1)–Fe(2) and Fe(2)–Fe(3) sites. The magnon dispersion relation derived from the linear spin wave approximation suggests the possible flat band nature of magnons. © 2021, The Author(s) This article is licensed under a Creative Commons Attribution 4.0 International License.
- ItemMagnetism of classical pyrochlore antiferromagnet Na3Mn(CO3)2Cl(American Physical Society, 2020-03-03) Nawa, K; Okuyama, D; Avdeev, M; Nojiri, H; Yoshida, M; Ueta, D; Yoshizawa, H; Sato, TJPyrochlore antiferromagnets have attracted interests in terms of unconventional ground states and spin excitations owing to competing interactions. When its magnetism is dominated by classical spins coupled by Heisenberg interactions, a spin liquid state is expected as its ground state because of infinite degeneracy in the ground state (R. Moessner and J. T. Chalker, Phys. Rev. Lett. 80, 2929 (1998); Phys. Rev. B 58, 12049 (1998).). In this research, we report structural and magnetic properties together with low-temperature neutron diffraction patterns on a new pyrochlore antiferromagnet Na3Mn(CO3)2Cl. The structure of Na3Mn(CO3)2Cl is isotypic with that of the Co-analogue Na3Co(CO3)2Cl, which exhibits all-in-all-out magnetic order below 1.5 K (Z. Fu et al., Phys. Rev. B 87, 214406 (2013)). On the other hand, no magnetic Bragg peak indicating a magnetic order was detected down to 0.05 K in Na3Mn(CO3)2Cl. A high degeneracy near the ground state is suggested by a magnetic entropy estimated from heat capacity experiments and enhancement of diffuse scattering from neutron diffraction experiments. © 2021 American Physical Society
- ItemPressure-induced superconductivity in the iron-based ladder material BaFe2S3(Springer Nature, 2015-07-20) Takahashi, H; Sugimoto, A; Nambu, Y; Yamauchi, T; Hirata, Y; Kawakami, T; Avdeev, M; Matsubayashi, K; Du, F; Kawashima, C; Soeda, H; Nakano, S; Uwatoko, Y; Ueda, Y; Sato, TJ; Ohgushi, KAll the iron-based superconductors identified so far share a square lattice composed of Fe atoms as a common feature, despite having different crystal structures. In copper-based materials, the superconducting phase emerges not only in square-lattice structures but also in ladder structures. Yet iron-based superconductors without a square-lattice motif have not been found, despite being actively sought out. Here, we report the discovery of pressure-induced superconductivity in the iron-based spin-ladder material BaFe2S3, a Mott insulator with striped-type magnetic ordering below ∼120 K. On the application of pressure this compound exhibits a metal–insulator transition at about 11 GPa, followed by the appearance of superconductivity below Tc = 14 K, right after the onset of the metallic phase. Our findings indicate that iron-based ladder compounds represent promising material platforms, in particular for studying the fundamentals of iron-based superconductivity. © 2015, Nature Publishing Group
- ItemSmall angle neutron scatterings study on the cubic chiral crystal Pr5Ru3Al2(International Conference on Neutron Scattering, 2017-07-12) Makino, K; Okuyama, D; Avdeev, M; Ohishi, K; Yamauchi, K; Oguchi, T; Sato, TJThe helical magnetic structure has attracted renewed interests because of the discovery of novel topological spin textures, for example magnetic skyrmions and chiral magnetic soliton lattices. For such spin textures, a finite antisymmetric Dzyaloshinskii-Moriya-type interaction is crucial, activated in noncentrosymmetric crystals. To date, such antisymmetric interactions have been studied mainly in 3d magnets, and few studies have been performed on 4f rare-earth (RE) magnets. Recently, Murashova et al. reported the RE-based chiral compounds RE5Ru3Al2 (RE = La, Ce, and Pr) with the space group I213. Nonetheless, their low-temperature magnetism was largely unexplored. Combining detailed magnetization and small-angle-neutron-scattering (SANS) measurements, we have scrutinized magnetic orderings in the Pr5Ru3Al2 compound at low temperatures under finite magnetic fields. In the magnetization study, we found at least four ordered phases in the ranges 1.9 < T< 3.8 K and 0 < H < 2500 Oe. The SANS study, performed using TAIKAN at J-PARC, revealed that under zero external field, two phases exists, characterized by the two distinct directions of their magnetic modulation vectors, q1 = (q q q): |q1| ~ 0.12 r. l. u. below 3.3 K, and q2 = (q q 0) : |q2| ~ |q1| observed for 3.3 K < T < 3.8 K. The magnetic modulation vectors under finite fields were similarly assigned. A first-principle electronic structure calculation has been made to understand those low-temperature ordered phases.