ANSTO :: Browsing by Author "Rosenfeld, AB"

Browsing by Author "Rosenfeld, AB"

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2nd generation microdosimeter with guard ring: an IBC study
(Australian Institute of Nuclear Science and Engineering (AINSE), 2009-11-25) Ziebell, AL; Hu, N; Lai, NS; Lim, WH; Reinhard, MI; Prokopovich, DA; Siegele, R; Dzurak, AS; Rosenfeld, AB
Silicon-on-insulator (SOI) micro dosimeters have recently been used to successfully measure the radiobiological properties of mixed radiation fields typical of medical, space and radiation protection environments. These SOI devices consist of a 2D array of elongated parallelepiped diode structures. Charge collection studies have revealed that due to the electric field distribution within the planar SV, there are significant lateral charge diffusion effects which complicate charge collection and give rise to a less than ideal chord length variance. © 2009 AINSE
3D radiation detectors: charge collection characterisation and applicability of technology for microdosimetry
(IEEE Xplore, 2014-08-04) Tran, LT; Prokopovich, DA; Petasecca, M; Lerch, MLF; Kok, A; Summanwar, A; Hansen, T; Via, CD; Reihnard, MI; Rosenfeld, AB
A study of charge collection in SINTEF 3D active edge silicon detectors was carried out at ANSTO using Ion Beam Induced Charge (IBIC) technique. An IBIC study has shown that several different geometries of 3D detectors have full depletion under low applied bias. The effect of fast neutron and gamma radiation on their charge collection efficiency was also investigated. A 3D active edge silicon detector technology has demonstrated extremely promising performance for application of the 3D Sensitive Volumes (SVs) fabrication methods to SOI microdosimetry.© 2014, IEEE.
3D sensitive volume microdosimeter with improved tissue equivalency: charge collection study and its application in 12C ion therapy
(IOP Publishing, 2018-02-06) James, B; Tran, LT; Bolst, D; Prokopovich, DA; Reinhard, MI; Lerch, MLF; Petasecca, M; Guatelli, S; Povoli, M; Kok, A; Matsufuji, N; Jackson, M; Rosenfeld, AB
This research focuses on the characterisation of a new 3D sensitive volume (SV) microdosimeter covered with polyimide – a material which closely mimics human tissue. The electrical and charge collection properties of the device were investigated and its application in 12C ion therapy were studied. Charge collection studies revealed uniform charge collection and no cross talk between adjacent SVs. To study the microdosimetric response in 12C ion therapy, the new polyimide mushroom microdosimeter were placed at various positions along the central axis of a 290 MeV/u 12C ion spread out Bragg peak (SOBP) at the Heavy Ion Medical Accelerator in Chiba (HIMAC), Japan. From these microdosimetric spectra, dose mean lineal energy $(\overline{{y}_{D})}$ and RBE10 results were obtained, with RBE10 increasing from 1.3 at the entrance to 2.7 at the end of the SOBP. The results obtained in this work show that the new generation of mushroom microdosimeters, covered with tissue equivalent polyimide material, are a useful tool for quality assurance in heavy ion therapy applications. © Open Access - CC BY - IOP Publishing Ltd.
Angular independent silicon detector for dosimetry in external beam radiotherapy
(American Association of Physicists in Medicine, 2015-07-17) Petasecca, M; Alhujaili, S; Aldosari, AH; Fuduli, I; Newal, M; Porumb, CS; Carolan, MG; Nitschke, K; Lerch, MLF; Kalliopuska, J; Perevertaylo, VL; Rosenfeld, AB
Purpose: In this work, the “edgeless” silicon detector technology is investigated, in combination with an innovative packaging solution, to manufacture silicon detectors with negligible angular response. The new diode is also characterized as a dosimeter for radiotherapy with the aim to verify its suitability as a single detector for in vivo dosimetry as well as large area 2D array that does not require angular correction to their response. Methods: For the characterisation of the “edgeless-drop-in” detector technology, a set of samples have been manufactured with different sensitive areas (1 × 1 and 0.5 × 0.5 mm2) and different thicknesses (0.1 and 0.5 mm) in four different combinations of top and peripheral p–n junction fabricated on p-type and n-type silicon substrates. The diode probes were tested in terms of percentage depth dose (PDD), dose rate, and linearity and compared to ion chambers. Measurements of the output factor have been compared to film. The angular response of the diodes probes has been tested in a cylindrical PMMA phantom, rotated with bidirectional accuracy of 0.25° under 10 × 10 cm2 6 MV Linac photon beam. The radiation hardness has been investigated as well as the effect of radiation damage on the angular and dose rate response of the diode probes when irradiated with photons from a Co-60 gamma source up to dose of 40 kGy. Results: The PDDs measured by the edgeless detectors show an agreement with the data obtained using ion chambers within ±2%. The output factor measured with the smallest area edgeless diodes (0.5 × 0.5 mm2—0.1 and 0.5 mm thick) matches EBT3 film to within 2% for square field size from 10 to 0.5 cm side equivalent distance. The dose rate dependence in a dose per pulse range of 0.9 × 10−5–2.7 × 10−4 Gy/pulse was less than −7% and +300% for diodes fabricated on p-type and n-type substrates, respectively. The edgeless diodes fabricated on the p-type substrate demonstrated degradation of the response as a function of the irradiation dose within 5%–15%, while diodes on the n-type substrate show a variation of approximately 30% after 40 kGy. The angular response of all probes is minimal (within 2%) but the N on N and P on P configurations show the best performances with an angular dependence of ±1.0% between 0° and 180° in the transversal direction. In this configuration, the space charge region of the passive diode extends from the behind and sidewall toward the anode on the top providing beneficial electric field distribution in the peripheral area of the diode. Such performance has also been tested after irradiation by Co-60 up to 40 kGy with no measurable change in angular response. Conclusions: A new edgeless-drop-in silicon diode fabrication and packaging technology has been used to develop detectors that show no significant angular dependence in their response for dosimetry in radiation therapy. From the characterisation of the diodes, proposed in a wide range of different geometries and configurations, the authors recommend the P-on-P detectors in conjunction with “drop in” packaging technology as the candidate for further development as single diode probe or 2D diode array for dosimetry in radiotherapy. © 2015 American Association of Physicists in Medicine
Characterisation of a well-type NaI(T1) detector by means of a Monte Carlo simulation for radionuclide metrology application
(Elsevier B. V., 2021-10) Heranudin, H; Smith, ML; van Wyngaardt, WM; Guatelli, S; Li, E; Rosenfeld, AB
A well-type NaI(Tl) detector was modelled and characterised by means of a Monte Carlo simulation, as part of a project to develop a 4πβ (Plastic Scintillator)-4πγ instrument to be used for the primary standardisation of radionuclides at ANSTO. The simulation based on GEANT4 was used to characterise the 4πγ detector in terms of potential dead layer/inactive materials, full energy peak efficiency, coincidence-summing correction, and energy resolution. An excellent agreement was obtained between the simulation results and the experimental measurements. © 2021 Elsevier Ltd.
Characterisation of a ΔE–E particle telescope using the ANSTO heavy ion microprobe
(Elsevier, 2007-07) Siegele, R; Reinhard, MI; Prokopovich, DA; Ionescu, M; Cohen, DD; Rosenfeld, AB; Cornelius, IM; Wroe, A; Lerch, MLF; Fazzi, A; Pola, A; Agosteo, S
Semiconductor planar processing technology has spurned the development of novel radiation detectors with applications in space, high energy physics, medical diagnostics, radiation protection and cancer therapy. The ANSTO heavy ion microprobe, which allows a wide range of ions to be focused into spot sizes of a few micrometers in diameter, has proven to be an essential tool for characterising these detectors using the Ion Beam Induced Charge (IBIC) imaging technique. The use of different ions and the wide range of available energies on the heavy ion microprobe, allows the testing of these devices with ionising particles associated with different values of linear energy transfer (LET). Quadruple coincidence measurements have been used to map the charge collection characteristics of a monolithic ΔE-E telescope, This was done through simultaneous measurement of the spatial coordinates of the microbeam relative to the sample and the response of both detector elements. The resulting charge collection maps were used to better understand the functionality of the device as well as to ascertain ways in which future device designs could be modified to improve performance. © 2007, Elsevier Ltd.
Characterization of prompt gamma rays for in-vivo range verification in hadron therapy: a geant4 simulation study
(Institute of Physics Publishing, 2018-02-06) Zarifi, M; Guatelli, S; Qi, Y; Bolst, D; Prokopovich, DA; Rosenfeld, AB
Prompt gamma (PG) rays have been proposed for in-vivo beam range verification during treatment delivery. As a secondary by-product emitted almost instantaneously upon ion-nuclear interaction, PG rays offer real-time tracking of the Bragg peak (BP). However their detection is challenging since they have a broad energy spectrum with interference from neutrons and stray gamma rays. Numerous approaches have been proposed to utilise PG for in-vivo beam range verification. In this work, Geant4 Monte Carlo (MC) simulations have been used to study the spectral, spatial, temporal and angular distribution characteristics of PG emission and detection from hadron radiation fields of varying energy. Proton, 12C and 4He beams irradiated homogeneous water phantoms. These studies will provide valuable information for the development of clinically suitable and reliable PG detector systems. © The Authors. Open Access.
Charge collection in SOI microdosimeters and their radiation hardness
(IEEE, 2023-02-03) Pan, VA; Tran, LT; Pastuovic, Z; Hill, D; Williams, JB; Kok, A; Povoli, M; Pogossov, A; Peracchi, S; Boardman, DA; Davis, J; Guatelli, S; Petasecca, M; Lerch, MLF; Rosenfeld, AB
A new batch of microdosimeters has been extensively studied for their charge collection efficiency (CCE) properties, as well as their radiation hardness for medical, space and accident applications. Silicon-on-insulator (SOI) microdosimeters with an active layer thickness of 10, 20 and 50 μm have been investigated and were characterized with a 24 MeV carbon ion beam as well as a Co-60 gamma source. A negative pulse was observed in addition to the positive pulses generated within the sensitive volumes (SVs) by incident ions which led to undesirable low energy events in the SOI microdosimeters response. To study this phenomenon, the microdosimeters were irradiated with gamma radiation from a Co-60 source with a total dose of 3 and 10 Mrad(Si). It was determined that the negative pulse was originating from the support wafer due to the displacement current phenomenon. Irradiation with the Co-60 source led to a disappearing of the negative pulse due to an increase in recombination within the support wafer while almost no changes in CCE were observed. A radiation hardness study was also performed on the 50 μm SOI microdosimeter with 16 SVs being irradiated with a fluence of ~ 10 8 12 C ions/cm 2 . A CCE deficit of approximately 2% was observed at an operation bias of 10V within the SVs. The findings of this work demonstrate that the SOI microdosimeters can be utilized in space and medical applications as they can handle typical levels of dose encountered in these applications. Additionally, evidence for SOI microdosimeter fabrication standards in terms of support wafer resistivity and buried oxide (BOX) thickness is shown. © 2023 IEEE
Comparison of SOI microdosimeter and tissue equivalent proportional counter measurements at the CERF facility
(Institute of Electrical and Electronics Engineers (IEEE), 2010-01-29) Prokopovich, DA; Reinhard, MI; Taylor, GC; Hands, A; Rosenfeld, AB
The CERN-EU High Energy Reference Field (CERF) facility is used in the calibration of neutron dosimeters for aviation and high energy physics applications. A comparison of the facility's microdosimetric spectra obtained with a new Silicon on Insulator (SOI) Microdosimeter and a HAWK Tissue Equivalent Proportional Counter (TEPC) are presented. Experimental measurements with a silicon PIN dosimeter diode are also described which indicate a small but significant contribution from charged particles to dosimetry measurements within the neutron dominated field.
Cylindrical silicon-on-insulator microdosimeter: charge collection characteristics.
(Australian Institute of Nuclear Science and Engineering (AINSE), 2007-11-22) Ziebell, AL; Lim, WH; Reinhard, MI; Cornelius, IM; Prokopovich, DA; Siegele, R; Dzurak, AS; Rosenfeld, AB
At present there exists a need, in both medical physics and radiation protection, for a portable microdosimeter that can be used in determining the radiobiological effectiveness (RBE) of different mixed radiation fields.
Cylindrical silicon-on-insulator microdosimeter: design, fabrication and TCAD modeling
(Institute of Electrical and Electronics Engineers (IEEE), 2009-04) Lim, WH; Ziebell, AL; Cornelius, IM; Reinhard, MI; Prokopovich, DA; Dzurak, AS; Rosenfeld, AB
A novel silicon-on-insulator (SOI) microdosimeter has been designed and fabricated using planar processing techniques to realise a device with a micron-scale well-defined sensitive volume. Cylindrical structures were employed to allow for an improved definition of the average chord length of the sensitive volume over that of previous elongated parallelepiped solid-state detector designs. The structures were manufactured on individual silicon mesas situated on top of a buried oxide insulating layer. The mesa design eliminated lateral charge diffusion. Two kinds of test structures were designed with sensitive region widths of 2 mum and 10 mum. In addition, an array of 900 cylindrical diodes was fabricated to increase the charge collection statistics. TCAD (Technology Computer Aided Design) modeling of the electrostatic potential and electric field profile of the cylindrical microdosimeter was carried out to obtain 3D potential and electric field profiles. The modeling revealed a radial electric field within the cylindrical-shaped sensitive volume with a 1/r dependence. While the electric field at the core of the cylindrical microdosimeter was not sufficiently high to induce avalanche signal multiplication, the higher electric field at the core should still assist in the measurement of low linear-energy transfer (LET) events. © 2009, Institute of Electrical and Electronics Engineers (IEEE)
Detection and discrimination of neutron capture events for NCEPT dose quantification
(Springer Nature Limited, 2022-04-07) Chacon, A; Kielly, M; Rutherford, H; Franklin, DR; Caracciolo, A; Buonanno, L; D'Adda, I; Rosenfeld, AB; Guatelli, S; Carminati, M; Fiorini, C; Safavi-Naeini, M
Neutron Capture Enhanced Particle Therapy (NCEPT) boosts the effectiveness of particle therapy by capturing thermal neutrons produced by beam-target nuclear interactions in and around the treatment site, using tumour-specific 10B or 157Gd-based neutron capture agents. Neutron captures release high-LET secondary particles together with gamma photons with energies of 478 keV or one of several energies up to 7.94 MeV, for 10B and 157Gd, respectively. A key requirement for NCEPT’s translation is the development of in vivo dosimetry techniques which can measure both the direct ion dose and the dose due to neutron capture. In this work, we report signatures which can be used to discriminate between photons resulting from neutron capture and those originating from other processes. A Geant4 Monte Carlo simulation study into timing and energy thresholds for discrimination of prompt gamma photons resulting from thermal neutron capture during NCEPT was conducted. Three simulated 300×300×300 mm3 cubic PMMA targets were irradiated by 4He or 12C ion beams with a spread out Bragg peak (SOBP) depth range of 60 mm; one target is homogeneous while the others include 10×10×10 mm3 neutron capture inserts (NCIs) of pure 10B or 157Gd located at the distal edge of the SOBP. The arrival times of photons and neutrons entering a simulated 50×50×50 mm3 ideal detector were recorded. A temporal mask of 50–60 ns was found to be optimal for maximising the discrimination of the photons resulting from the neutron capture by boron and gadolinium. A range of candidate detector and thermal neutron shielding materials were simulated, and detections meeting the proposed acceptance criteria (i.e. falling within the target energy window and arriving 60 ns post beam-off) were classified as true or false positives, depending on their origin. The ratio of true/false positives (RTF) was calculated; for targets with 10B and 157Gd NCIs, the detector materials which resulted in the highest RTF were cadmium-shielded CdTe and boron-shielded LSO, respectively. The optimal irradiation period for both carbon and helium ions was 1 µs for the 10B NCI and 1 ms for the 157Gd NCI. © The Authors, Creative Commons Attribution 4.0 International Licence.
Development and fabrication of cylindrical silicon-on-insulator microdosimeter arrays.
(Institute of Electrical and Electronics Engineers (IEEE), 2009-06) Lai, NS; Lim, WH; Ziebell, AL; Reinhard, MI; Rosenfeld, AB; Dzurak, AS
Recent developments in the fabrication and simulation of prototype silicon-on-insulator (SOI) microdosimeter arrays are presented. A new planar array design has been proposed which has a number of advantages over the previous elongated parallelepiped and cylindrical mesa array designs. This novel planar array design, which incorporates a guard ring, is based upon 2500 planar cylindrically shaped p-i-n detectors and was fabricated via dopant diffusion and ion implantation. The dopant-diffused arrays were successfully fabricated and tested using 2 mum and 10-mum- thick SOI substrates. Technology computer-aided design modeling of the ion-implanted structure is presented which includes the electrostatic potential profile, showing possible avalanche signal multiplication around the n+ core of the microdosimeter. The alpha particle charge transient response was simulated to determine the charge collection in the sensitive region. © 2009, Institute of Electrical and Electronics Engineers (IEEE)
Development of a large-area silicon α-particle detector
(Elsevier, 2014-09) Tran, LT; Prokopovich, DA; Lerch, MLF; Petasecca, M; Siegele, R; Reinhard, MI; Perevertaylo, VL; Rosenfeld, AB
Circular ion-implanted silicon detector of α-particles with a large, 5-cm2, sensitive area has been developed. An advantage of the detector is that the detector surface is easily cleanable with chemicals. The hardened surface of the detector shows no signs of deterioration of the spectroscopic and electrical characteristics upon repeated cleaning. The energy resolution along the diameters of the detector was (1.0±0.1)% for the 5.486-MeV α-particles. Detailed tests of the charge collection efficiency and uniformity of the detector entrance window were also performed with a 5.5-MeV He2+ microbeam. © 2014, Elsevier Ltd.
Development of LEU-based targets for radiopharmaceutical manufacturing: a review
(Elsevier, 2019-06) Raposio, R; Thorogood, GJ; Czerwinski, K; Rosenfeld, AB
99Mo is an essential medical isotope that comprises of at least 70% of radioactive procedures globally. Currently an essential component of 99Mo manufacturing is the uranium target from which 99Mo is produced by fission. As the world moves towards low enriched uranium (LEU) targets due to non-proliferation concerns it is becoming of interest to find methods to increase the efficiency of the LEU targets in order to reduce the ever increasing nuclear waste levels of which a long term solution for disposal or treatment has yet to be satisfactorily found. Advantages and disadvantages of various target designs are investigated and discussed along current disposal and reprocessing methods. The idea of a reusable target is introduced as a way forward in reducing the nuclear waste burden for future generations. © 2019 Elsevier Ltd.
Evaluation of silicon detectors with integrated JFET for biomedical applications
(Institute of Electrical and Electronics Engineers (IEEE), 2009-06) Safavi-Naeini, M; Franklin, DR; Lerch, MLF; Petasecca, M; Pignatel, G; Reinhard, MI; Dalla Betta, GF; Zorzi, N; Rosenfeld, AB
This paper presents initial results from electrical, spectroscopic and ion beam induced charge (IBIC) characterisation of a novel silicon PIN detector, featuring an on-chip n -channel JFET and matched feedback capacitor integrated on its p-side (frontside). This structure reduces electronic noise by minimising stray capacitance and enables highly efficient optical coupling between the detector back-side and scintillator, providing a fill factor of close to 100%. The detector is specifically designed for use in high resolution gamma cameras, where a pixellated scintillator crystal is directly coupled to an array of silicon photodetectors. The on-chip JFET is matched with the photodiode capacitance and forms the input stage of an external charge sensitive preamplifier (CSA). The integrated monolithic feedback capacitor eliminates the need for an external feedback capacitor in the external electronic readout circuit, improving the system performance by eliminating uncontrolled parasitic capacitances. An optimised noise figure of 152 electrons RMS was obtained with a shaping time of 2 mus and a total detector capacitance of 2 pF. The energy resolution obtained at room temperature (2°C) at 27 keV (direct interaction of I-125 gamma rays) was 5.09%, measured at full width at half maximum (FWHM). The effectiveness of the guard ring in minimising the detector leakage current and its influence on the total charge collection volume is clearly demonstrated by the IBIC images. © 2009, Institute of Electrical and Electronics Engineers (IEEE)
First extensive study of silver-doped lanthanum manganite nanoparticles for inducing selective chemotherapy and radio-toxicity enhancement
(Elsevier B. V., 2021-04) Khochaiche, A; Westlake, M; O'Keefe, A; Engels, E; Vogel, S; Valceski, M; Li, N; Rule, KC; Horvat, J; Konstantinov, K; Rosenfeld, AB; Lerch, MLF; Corde, S; Tehei, M
Nanoparticles have a great potential to increase the therapeutic efficiency of several cancer therapies. This research examines the potential for silver-doped lanthanum manganite nanoparticles to enhance radiation therapy to target radioresistant brain cancer cells, and their potential in combinational therapy with magnetic hyperthermia. Magnetic and structural characterisation found all dopings of nanoparticles (NPs) to be pure and single phase with an average crystallite size of approximately 15 nm for undoped NPs and 20 nm for silver doped NPs. Additionally, neutron diffraction reveals that La0.9Ag0.1MnO3 (10%-LAGMO) NPs exhibit residual ferromagnetism at 300 K that is not present in lower doped NPs studied in this work, indicating that the Curie temperature may be manipulated according to silver doping. This radiobiological study reveals a completely cancer-cell selective treatment for LaMnO3, La0.975Ag0.025MnO3 and La0.95Ag0.05MnO3 (0, 2.5 and 5%-LAGMO) and also uncovers a potent combination of undoped lanthanum manganite with orthovoltage radiation. Cell viability assays and real time imaging results indicated that a concentration of 50 μg/mL of the aforementioned nanoparticles do not affect the growth of Madin-Darby Canine Kidney (MDCK) non-cancerous cells over time, but stimulate its metabolism for overgrowth, while being highly toxic to 9L gliosarcoma (9LGS). This is not the case for 10%-LAGMO nanoparticles, which were toxic to both non-cancerous and cancer cell lines. The nanoparticles also exhibited a level of toxicity that was regulated by the overproduction of free radicals, such as reactive oxygen species, amplified when silver ions are involved. With the aid of fluorescent imaging, the drastic effects of these reactive oxygen species were visualised, where nucleus cleavage (an apoptotic indicator) was identified as a major consequence. The genotoxic response of this effect for 9LGS and MDCK due to 10%-LAGMO NPs indicates that it is also causing DNA double strand breaks within the cell nucleus. Using 125 kVp orthovoltage radiation, in combination with an appropriate amount of NP-induced cell death, identified undoped lanthanum manganite as the most ideal treatment. Real-time imaging following the combination treatment of undoped lanthanum manganite nanoparticles and radiation, highlighted a hinderance of growth for 9LGS, while MDCK growth was boosted. The clonogenic assay following incubation with undoped lanthanum manganite nanoparticles combined with a relatively low dose of radiation (2 Gy) decreased the surviving fraction to an exceptionally low (0.6 ± 6.7)%. To our knowledge, these results present the first biological in-depth analysis on silver-doped lanthanum manganite as a brain cancer selective chemotherapeutic and radiation dose enhancer and as a result will propel its first in vivo investigation. © 2021 Elsevier B.V.
From imaging to dosimetry: GEANT4-based study on the application of medipix to neutron dosimetry
(Elsevier, 2009-10-12) Othman, MAR; Marinaro, DG; Petasecca, M; Guatelli, S; Cutajar, DL; Lerch, MLF; Prokopovich, DA; Reinhard, MI; Uher, J; Jakubek, J; Pospisil, S; Rosenfeld, AB
An application of Medipix2 using a newly developed segmented multiple thickness polyethylene (PE) converter for fast neutron detection is presented. The system has the ability to provide an energy independent response for the dose equivalent for fast neutrons. The application of weighting factors to each defined thickness of PE allows for a flattening of the response of the detector system for dosimetry applications. Six PE converter segments were applied, and their thicknesses and weighting factors were optimised to obtain the required energy independent detector response. The study performed by means of GEANT4. Its suitability for neutron dosimetry was studied with respect to a previously published work. © 2013 Elsevier B.V.
Geant4 simulation of the CERN-EU high-energy reference field (CERF) facility
(Oxford University Press (OUP), 2010-09) Prokopovich, DA; Reinhard, MI; Cornelius, IM; Rosenfeld, AB
The CERN-EU high-energy reference field facility is used for testing and calibrating both active and passive radiation dosemeters for radiation protection applications in space and aviation. Through a combination of a primary particle beam, target and a suitable designed shielding configuration, the facility is able to reproduce the neutron component of the high altitude radiation field relevant to the jet aviation industry. Simulations of the facility using the GEANT4 (GEometry ANd Tracking) toolkit provide an improved understanding of the neutron particle fluence as well as the particle fluence of other radiation components present. The secondary particle fluence as a function of the primary particle fluence incident on the target and the associated dose equivalent rates were determined at the 20 designated irradiation positions available at the facility. Comparisons of the simulated results with previously published simulations obtained using the FLUKA Monte Carlo code, as well as with experimental results of the neutron fluence obtained with a Bonner sphere spectrometer, are made. © 2010, Oxford University Press (OUP)
Geant4 x-ray fluorescence with updated libraries
(Elsevier B. V., 2021-11-15) Bakr, S; Cohen, DD; Siegele, R; Archer, JW; Incerti, S; Ivanchenko, V; Mantero, A; Rosenfeld, AB; Guatelli, S
We present the results concerning the development in Geant4 of a new data driven library, called here the ANSTO HF library. This X-ray fluorescence library is based on an approach of particular interest for PIXE simulation applications; however, it can be used in any Geant4 applications where X-ray fluorescence needs to be described. The X-ray fluorescence transition probabilities were calculated within the Hartree-Fock (HF) approach, which is recognised to better reproduce PIXE experimental values compared with the Hartree-Slater approach, adopted in the current default Geant4 EADL data library. These HF X-ray fluorescence transition probabilities were integrated into a new Geant4 library and will be released within Geant4 in the near future. In this paper, we compare the fluorescence X-ray spectra generated by the ANSTO HF library and by the currently available library (EADL-1991 [1]) within Geant4, for targets irradiated with protons and α particles with energies up to 10 MeV, a range of interest for PIXE applications. The comparisons were performed for a large set of sample materials spanning a broad range of target atomic numbers. These two approaches were compared to existing experimental measurements performed at the ANSTO heavy ion microprobe beamline using 2 MeV and 3 MeV proton and 10 MeV He2+ ion beams. This work represents a useful upgrade to the Geant4 atomic de-excitation package. © 2021 Elsevier B.V.

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