Browsing by Author "Jain, A"

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    Competing exchange interactions on the verge of a metal-insulator transition in the two-dimensional spiral magnet Sr3Fe2O7
    (Americal Physical Society, 2014-10-03) Kim, JH; Jain, A; Reehuis, M; Khaliullin, G; Peets, DC; Ulrich, C; Park, JT; Faulhaber, E; Hoser, A; Walker, HC; Adroja, DT; Walters, AC; Inosov, DS; Maljuk, A; Keimer, B
    We report a neutron scattering study of the magnetic order and dynamics of the bilayer perovskite Sr 3 Fe 2 O 7 , which exhibits a temperature-driven metal-insulator transition at 340 K. We show that the Fe 4+ moments adopt incommensurate spiral order below T N =115  K and provide a comprehensive description of the corresponding spin-wave excitations. The observed magnetic order and excitation spectra can be well understood in terms of an effective spin Hamiltonian with interactions ranging up to third-nearest-neighbor pairs. The results indicate that the helical magnetism in Sr 3 Fe 2 O 7 results from competition between ferromagnetic double-exchange and antiferromagnetic superexchange interactions whose strengths become comparable near the metal-insulator transition. They thus confirm a decades-old theoretical prediction and provide a firm experimental basis for models of magnetic correlations in strongly correlated metals. © 2014, American Physical Society.