ANSTO :: Browsing by Author "Fink, D"

Browsing by Author "Fink, D"

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10Be and 26Al exposure history of the highest mountains in Wales: evidence from Snowdon and the Glyders
(International Union for Quaternary Research (INQUA), 2019-07-28) Hughes, PD; Glasser, NF; Fink, D
Cosmogenic 10Be and 26Al exposure ages from samples collected from the mountains of Glyders (1001 m) and from Snowdon (1085 m) in Wales provide new insights into the glacial history of the highest mountains in the British Isles outside of Scotland. Sample elevations range from 598 to 1013 m and taken from centimetre-thick quartz veins on bedrock and also one boulder. The summits of the Glyders are characterised by intensely modified frost-shattered surfaces and have long been recognised as exemplars of mountain summit periglacial activity in the British Isles. However, numerous glacially-transported boulders on the highest ground indicate that ice overran the summits. Bedrock samples at c. 960 m yielded 10Be exposure ages of 72 ka and 153 ka. In addition, a glacially-transported boulder at 985 m gave a 10Be age of 57 ka. This boulder sample is important because it negates issues of inheritance that are possible with bedrock samples and it provides the closest estimate of the timing of ice thinning and the true exposure age of the Glyders summits. All 26Al ages were consistent indicating non-complex histories. These results clearly confirm the Glyder summits were overtopped by the Welsh Ice Cap during marine isotope stage (MIS) 4, when ice in this area was thicker than at the global last glacial maximum (LGM) in MIS 2. The summits were revealed as ice thinned during the transition from MIS 4 to 3. Both the geomorphological evidence and our new cosmogenic ages support recent ice cap modelling predictions that the summits then stood as nunataks above the LGM ice sheet surface in MIS 2. The oldest 10Be (and 26Al) age of ~150 ka from the frost-shattered summit tor displays significant nuclide inheritance and previous work has demonstrated evidence of gibbsite in the summit soils. The wide range in 10Be apparent exposure ages and the evidence of glacially-transported boulders on intensely frost-shattered bedrock suggests erosion of the Glyder summit surfaces largely proceeded by plucking/quarrying rather than abrasion. This would have occurred under cold-based conditions with ice flow dominated by internal deformation rather than sliding. In contrast, at altitudes below 900 m ice-scoured rock surfaces on both the Glyders and neighbouring Snowdon yield exposure ages consistent with deglaciation after the global LGM in MIS 2. Based on these ages and similar results from other summits in North Wales the Welsh Ice Cap rapidly thinned after c. 20 ka leading to a phase of alpine-style glaciation. However, on Snowdon, arête crests yielded very young apparent ages of ~ 5 ka. These young ages reflect continual stripping of the arête rock surfaces through the current interglacial.
10Be concentrations in snow at Law Dome, Antarctica following the 29 October 20 and 20 January 2005 solar cosmic ray events
(World Scientific, 2009-08) Pedro, JB; Smith, AM; Duldig, ML; Klekociuk, AR; Simon, KJ; Curran, MAJ; van Ommen, TD; Fink, D; Morgan, VI; Galton-Fenzi, BK
Recent model calculations have attempted to quantify the contribution of major energetic solar cosmic ray (SCR) events to 10Be production.1,2 In this study we compare modeled 10Be production by SCR events to measured 10Be concentrations in a Law Dome snow pit record. The snow pit record spans 2.7 years, providing a quasi-monthly 10Be sampling resolution which overlaps with the SCR events of 29 Oct 2003 and 20 Jan 2005. These events were calculated to increase monthly 10Be production in the polar atmosphere (>65° S geomagnetic latitude) by ~60% and ~120% above the GCR background, respectively2. A strong peak in 10Be concentrations (>4σ above the 2.7 y mean value) was observed ~1 month after the 20 Jan 2005 event. By contrast, no signal in 10Be concentrations was observed following the weaker 29 Oct 2003 series of events. The concentration of 10Be in ice core records involves interplay between production, transport, and deposition processes. We used a particle dispersion model to assess vertical and meridional transport of aerosols from the lower stratosphere where SCR production of 10Be is expected to occur, to the troposphere from where deposition to the ice sheet occurs. Model results suggested that a coherent SCR production signal could be transported to the troposphere within weeks to months following both SCR events. We argue that only the 20 Jan 2005 SCR event was observed in measured concentrations due to favorable atmospheric transport, relatively high production yield compared to the 29 Oct 2003 event, and a relatively high level of precipitation in the Law Dome region in the month following the event. This result encourages further examination of SCR signals in 10Be ice core data. © 2009 World Scientific Publishing
10Be exposure ages of ancient desert pavements reveal Quaternary evolution of the Dead Sea drainage basin and rift margin tilting
(Elsevier, 2010-02-15) Guralnik, B; Matmon, A; Avni, Y; Fink, D
Early to late Pleistocene 10Be exposure ages of abandoned surfaces in the Negev desert reveal the regional drainage evolution history and its relationship with the subsidence of the western margin of the Dead Sea Rift. The dated desert paved surfaces have developed over originally westward-flowing rivers, which were abandoned by early Pleistocene and whose relicts are now progressively tilted towards the rift axis. The slow and non-destructive subsidence coupled with extreme hyperaridity enabled the preservation of these ancient surfaces along some of the main water divides in the Negev, nearly irrespective of their distance from the rift axis. Constraints on the tilting history are obtained from analyzing the spatial pattern of the exposure ages, suggesting subsidence rates as low as 120–300 m Ma–1 in the southern Arava Valley since the late Pliocene. It is shown that the transition from the Pliocene to current drainage pattern occurred over a short period during the early Pleistocene, and that the governing fluvial response that followed the delineation of current basins is represented by a continuous spectrum of ages of inset terraces.
14C AMS measurements of the bomb pulse in N- and S- hemisphere tropical trees
(Elsevier, 1997-03-02) Murphy, JO; Lawson, EM; Fink, D; Hotchkis, MAC; Hua, Q; Jacobsen, GE; Smith, AM; Tuniz, C
The 14C bomb-pulse signature has been measured by AMS on cross-dateable teak samples from N- and S-hemisphere locations in the tropics. Excellent agreement is found with the atmospheric 14C content in the period 1955 to 1980 for the respective hemispheres. These results demonstrate that 14C measurements can be used to facilitate growth rate determinations in tropical trees. © 1997 Elsevier B.V.
14C analyses at the ANTARES AMS Centre: dating the log coffins of northwest Thailand
(Elsevier, 1994-06-03) Hotchkis, MAC; Fink, D; Jacobsen, GE; Lawson, EM; Shying, ME; Smith, AM; Tuniz, C; Barbetti, M; Grave, P; Quan, HM; Head, J
Recent results of 14C analyses at the ANTARES AMS Centre are presented. Test measurements of 14C blanks demonstrate an ultimate sensitivity of the order of 10−15 (14C/12C ratio). Measurements of unknowns have been made with a precision in the range 1–1.5% using a “slow cycling” mode of operation where the injection magnet field is changed to inject 14C and 13C alternately. Results are presented for a series of log coffins from cave burials in NW Thailand. © 1994 Elsevier B.V.
14C in uranium and thorium minerals: a signature of cluster radioactivity?
(Springer Nature, 1999-06-01) Bonetti, R; Guglielmetti, A; Poli, G; Sacchi, E; Fink, D; Hotchkis, MAC; Jacobsen, GE; Lawson, EM; Hua, Q; Smith, AM; Tuniz, C
Various uranium and thorium minerals have been analysed with accelerator mass spectrometry to determine their 14C content. It is found that, whenever the contribution from secondary reactions such as the 11B(α,p)14C is sufficiently low, the 14C concentration is consistent with that expected from 14C (spontaneous) cluster radioactivity from radium isotopes of the uranium and thorium natural series. © Springer-Verlag 1999
15th International Conference on Accelerator Mass Spectrometry
(Australian Nuclear Science and Technology Organisation, 2021-11-15) Bertuch, F; Child, DP; Fink, D; Fülöp, RH; Hotchkis, MAC; Hua, Q; Jacobsen, GE; Jenkinson, A; Levchenko, VA; Simon, KJ; Smith, AM; Wilcken, KM; Williams, AA; Williams, ML; Yang, B; Fallon, SJ; Wallner, T
On behalf of the AMS-15 Organising committee, we would like to thank you for attending the 15th International Conference on Accelerator Mass Spectrometry. Held as an online event for the first time, the 2021 conference attracted over 300 attendees with presentations delivered by colleagues and professionals from around the globe.Applications of AMS to the world’s most pressing problems/questions: A-1 : Earth’s dynamic climate palaeoclimate studies, human impacts on climate, data for climate modelling. A-2 : Water resource sustainability groundwater dating, hydrology, water quality and management A-3 : Living landscapes soil production, carbon storage, erosion, sediment transport, geomorphology. A-4 : Catastrophic natural events volcanoes, cyclones, earthquakes, tsunamis, space weather, mass extinctions. A-5 : Advancing human health metabolic and bio-kinetic studies, bomb-pulse dating, diagnostics and bio-tracing. A-6 : Challenges of the nuclear age nuclear safeguards, nuclear forensics, nuclear waste management, nuclear site monitoring, impacts of nuclear accidents. A-7 :Understanding the human story archaeology, human evolution and migration, history, art and cultural heritage A-8 : Understanding the cosmos fundamental physics, nuclear astrophysics, nuclear physics AMS Research and Development: T-1 : Novel AMS systems, components and techniques T-2 : Suppression of isobars and other interferences T-3 : Ion sourcery T-4 : New AMS isotopes T-5 : Advances in sample preparation T-6 : Data quality and management T-7 : Facility Reports (Poster Presentation only)
A 2 million year glacial chronology of the Hatherton Glacier, Antarctica and implications for the size of the East Antarctic Ice Sheet at the Last Glacial Maximum
(Pergamon-Elsevier Science Ltd, 2014-01-01) Joy, K; Fink, D; Storey, BC; Atkins, C
A series of distinct glacial deposits flanking the margins of the upper Hatherton Glacier, an outlet glacier in the central Transantarctic Mountains, are used to constrain the behaviour of the Antarctic ice-sheets. Cosmogenic exposure ages of 18 erratics from four glacial drifts covering the ice free Dubris and Bibra valleys, range in age from 5 to 1997 ka. Our results document four glacial advance and retreat events superimposed on an overall long-term ice thickness reduction of about 500 m since the mid-Pleistocene. The lack of field evidence and absence of LGM exposure ages in the glacial deposits of the Hatherton Glacier supports our conclusion that at the LGM the East Antarctic Ice Sheet was of similar size, or may have been slightly smaller, than present. Minimum exposure ages from the oldest two glacial events, represented by the Isca and Danum drifts, are similar to 1-2 Ma and similar to 0.5 Ma respectively. The Britannia-II Drift, previously assumed to mark the maximum extent of the Last Glacial Maximum advance, has a mean Be-10 age of 126 +/- 3.2 ka (n = 5). Ages from the younger Britannia-I Drift suggest that since the mid-Holocene (6.5 +/- 1.2 ka, n = 5), approximately 200 m of additional ice has been lost. © 2014, Elsevier Ltd.
21Ne, 10Be and 26Al cosmogenic burial ages of near-surface eolian sand from the Packard Dune field, McMurdo Dry Valleys, Antarctica
(XIX INQUA Congress "Quaternary Perspectives on Climate Change, Natural Hazards and Civilization", 2015-07-26) Fink, D; Augustinus, PC; Rhodes, E; Bristow, C; Balco, G
The McMurdo Dry Valleys, Antarctica, have been ice-free for at least 10 Ma. In Victoria Valley, the largest of the Dry Valleys, permafrosted yet still actively migrating dune-fields, occupy an area of 8 km2 with dune thicknesses varying from 5 to 70 meters. High-resolution ground penetrating radar (GPR) imaging of selected dunes reveal numerous unconformities and complex stratigraphy inferring cycles of sand accretion and deflation from westerly katabatic winter winds sourced from the East Antarctic Ice Sheet and anabatic summer winds sourced from the Ross Sea. Samples above permafrost depth were taken for OSL and cosmogenic 26Al/10Be burial ages. OSL ages from shallow (<1m) pits range from modern to 1.3ka suggesting that deposition/reworking of the dunes is ongoing and their present configuration is a late Holocene feature. The same 7 samples gave a mean 26Al/10Be = 4.53 +/- 5% with an average apparent continuous 10Be surface exposure age of 525 +/- 25 ka surprisingly indicating a common pre-history independent of depth. Correcting for minor post-burial production based on OSL ages, the minimum (integrated) burial period for these sand grains is 0.51+/- 0.12 Ma which represents the burial age at the time of arrival at the dune. A possible explanation is that this common burial signal reflects recycling episodes of exposure, deposition, burial and deflation, sufficiently frequent to move all grains towards a common pre-dune deposition history. However, it is unclear over what length of time this processes has been active and fraction of time the sand has been buried. Consequently we also analysed purified quartz aliquots of the same samples for a third and stable nuclide, 21Ne, to determine the total surface and burial exposure periods. Using the 21Ne/10Be system we obtain burial ages of 1.10 +/- 0.10 Ma. Further coring below permafrost is planned for austral summer 2015. © Copyright, 2015 XIX INQUA Congress LOC.
26Al/10Be dating of an aeolian dust mantle soil in western New South Wales, Australia
(Elsevier B.V., 2014-08-15) Fisher, A; Fink, D; Chappell, JMA; Melville, MD
Aeolian dust mantle soils are an important element of many landscapes in south-eastern Australia, though the age of these aeolian deposits has not been radiometrically determined. At Fowlers Gap in western New South Wales, surface cobbles of silcrete and quartz overlie a stone-free, aeolian dust mantle soil, which has a thickness of about 1.6m. The clay-rich aeolian dust deposit in turn lies upon a buried silcrete and quartz stone layer. Modelling in-situ cosmogenic 26Al and 10Be concentrations measured in both the surface quartz stones and in the buried quartz layer of rocks, reveals that each has experienced a complex exposure-burial history. Due to the absence of quartz stones or sand at intermediate depths, our cosmogenic 26Al and 10Be modelling was not able to determine a definitive mechanism of stone pavement formation and stone burial. Various scenarios of stone formation, transport, burial and exhumation were tested that constrain the age of the deposit to range from 0.9±0.2Ma to 1.8±0.2Ma, based largely on different assumptions taken for the time-dependency of the net sedimentation rate. This corresponds with the initiation of the Simpson Desert dune fields and the deflation of lakes in central Australia, which probably responded to the shift to longer-wavelength, larger-amplitude Quaternary glacial cycles at around 1Ma. Sensitivity analyses were carried out to identify those parameters which better constrained model outputs. Within model errors, which largely are the result of analytical errors in measured 26Al and 10Be concentrations, all three competing theories of colluvial wash, upward displacement of stones, and cumulic pedogenesis are possible mechanisms for the formation of the surface stone pavement. © 2020 Elsevier B.V
26Al/10Be dating of an aeolian dust mantle soil in western New South Wales, Australia
(Australian Geosciences Council, 2012-08-05) Fisher, A; Fink, D; Chappell, JMA; Melville, MD
Aeolian dust mantle soils are an important element of many landscapes in southeastern Australia, though the age of the aeolian deposits has rarely been determined. Measuring 26Al and 10Be in rocks and cobbles buried by an aeolian dust mantle soil at Fowlers Gap in western New South Wales, and modelling their exposure history has revealed the age of the deposit to be 1.1 ± 0.2 Ma, placing increasing aridity at least back to MIS 22, many stages before the MIS 10 increase in aeolian dust observed within Tasman Sea cores. The aeolian age of 1Ma coincides with initiation of the Simpson Desert dunefields and deflation of lakes in central Australia, which likely responded to the shift to longer-wavelength larger-amplitude Quaternary glacial cycles at the mid-Pleistocene Transition. Modelling the 26Al and 10Be exposure history of samples from the surface stone pavement has shown that they have experienced periods of prolonged burial. The simplest explanation for this burial is that the surface cobbles were buried, perhaps episodically, during periods of aeolian deposition, before travelling upwards through the soil to be re-exposed at the new ground surface. Vertical stone movement may have occurred through soil heaving as clay minerals swell and shrink upon wetting and drying, evidence of which is visible in the gilgai-microtopography and horizontal stone sorting (patterned ground) at the site.
26Al/10Be ratios reveal the source of river sediments in the Kimberley, NW Australia
(Wiley, 2020-02-07) Cazes, G; Fink, D; Codilean, AT; Fülöp, RH; Fujioka, T; Wilcken, KM
We use cosmogenic 10Be and 26Al in both bedrock and fluvial sediments to investigate controls on erosion rates and sediment supply to river basins at the regional scale in the Kimberley, NW Australia. The area is characterised by lithologically controlled morphologies such as cuestas, isolated mesas and extensive plateaus made of slightly dipping, extensively jointed sandstones. All sampled bedrock surfaces at plateau tops, ridgelines, and in the broader floodplain of major rivers over the region show similar slow lowering rates between 0.17 and 4.88 m.Myr-1, with a mean value of 1.0 ± 0.6 m.Myr-1 (n=15), whilst two bedrock samples collected directly within river-beds record rates that are one to two orders of magnitude higher (14.4 ± 1.5 and 20.9 ± 2.5 m.Myr-1, respectively). Bedrock 26Al/10Be ratios are all compatible with simple, continuous sub-aerial exposure histories. Modern river sediment yield lower 10Be and 26Al concentrations, apparent 10Be basin-wide denudation rates ranging between 1.8 and 7.7 m.Myr-1, with a median value of 2.6 m.Myr-1, more than double the magnitude of bedrock erosion rates. 26Al/10Be ratios of the sediment samples are lower than those obtained for bedrock samples. We propose that these depleted 26Al/10Be ratios can largely be explained by the supply of sediment to river basins from the slab fragmentation and chemical weathering of channel gorge walls and plateau escarpments that result in diluting the cosmogenic nuclide concentration in river sediments measured at the basin outlets. The results of a mass-balance model suggest that ~60–90% of river sediment in the Kimberley results from the breakdown and chemical weathering of retreating vertical sandstone rock-walls in contrast to sediment generated by bedrock weathering and erosion on the plateau tops. This study emphasises the value of analysing two or more isotopes in basin-scale studies using cosmogenic nuclides, especially in slowly eroding post-orogenic settings. © 2019 John Wiley & Sons, Ltd.
36Cl exposure-age chronology of Late Pleistocene glaciations on Mount Tymphi, Pindus Mountains, northwest Greece
(International Union for Quaternary Research (INQUA), 2019-07-27) Allard, JL; Hughes, PD; Woodward, JC; Fink, D; Simon, KJ; Wilcken, KM
The mountains of Greece and the wider Balkans were glaciated during the Pleistocene. The most extensive glaciations occurred during the Middle Pleistocene when large ice caps and glaciers formed in several ranges including the Dinaric Alps and the Pindus Mountains. The Late Pleistocene in the Balkans, however, was characterised by smaller ice masses with glaciers restricted to the highest mountains. Nevertheless, these glaciers were important in shaping much of the high mountain landscapes that we see today and they supplied many rivers with outwash sediments. Here we present preliminary results from 36Cl terrestrial cosmogenic nuclide analyses. From samples collected in summer 2017, we have calculated exposure ages from moraine boulders and glaciated bedrock in the uppermost valleys and cirques of Mount Tymphi massif (2497 m) in northwest Greece. We address both a significant geographical gap in Mediterranean glacial chronologies and the temporal gap in the glacial history of this region by targeting the previously undated Late Pleistocene glacial record. Coupled with published U-series ages from lower elevation moraines, this is the first glacial chronology in the east-central Mediterranean based on multiple dating methods. On the southwest side of the massif, 18 exposure ages obtained from 3 moraines in the cirque and mouth of the Laccos Megalon Litharion valley and the mouth of the western cirque of Tsioumako (2155 m), indicate moraine formation between 1700 m and 2050 m a.s.l. during the Late Pleistocene. This complements previous U-series ages obtained from secondary calcites in glacial sediments below 1700 m (and elsewhere in the Balkans), which demonstrate more extensive glaciations dating to the Middle Pleistocene. At ~1430 m a.s.l. in the Laccos cirque on the northeast side of the massif, 6 exposure ages (5 boulders, 1 bedrock) from a pair of end moraines represent the first dates from this side of Mount Tymphi. They suggest small cirque glaciers persisted until at least the end of the Late Pleistocene, facilitated by avalanching snow and shading from the cliffs of Goura (2467 m). Understanding where, when and why glaciers reached their maxima during the last glacial cycle is not only important for understanding the dynamics of the glacial climate in this region, but also for the timing of sediment and meltwater delivery to river systems; the dynamics of Mediterranean refugia; and has implications for understanding the environmental context of nearby Middle and Upper Palaeolithic archaeological records.
41Ca, 26Al, and 10Be in lunar basalt 74275 and 10Be in the double drive tube 74002/74001
(Elsevier, 1998-07) Fink, D; Klein, J; Middleton, R; Vogt, S; Herzog, GF; Reedy, RC
We report depth profiles of the cosmogenic radionuclides 10Be, 26Al, and 41Ca in the titanium-rich lunar basalt 74275. The 10Be profile is flat: 10Be activities are confined to a narrow range between 9.6 and 11.2 dpm/kg but are nonetheless consistent with a small contribution of about 1–2 dpm/kg from solar cosmic rays. The 26Al profile shows the steep decrease with increasing depth that is characteristic of nuclides whose production is dominated by solar cosmic rays. 41Ca activities decrease from about 22 dpm/kg at the surface to a minimum of ∼9 dpm/kg at a depth of 4.7 g/cm2 and then increase to ∼11 dpm/kg at a depth of 15.8 g/cm2. The sharp decrease near the surface identifies for the first time production of 41Ca by solar cosmic rays. We also report 10Be measurements for six samples from lunar core 74002/1. The 10Be activities range from approximately 8 to 14 dpm/kg. We model the production of 10Be, 26Al, and 41Ca in lunar rock 74275 by including published data that indicate a long exposure to galactic cosmic rays at a depth of 140 g/cm2 followed by one at the surface lasting 2.8 Ma. Cosmogenic radionuclide production by galactic cosmic rays, and, in the case of 41Ca, by thermal neutrons is estimated from published measurements and semi-empirical calculations. Our model includes a new calculation of production rates due to solar cosmic rays and incorporates recently published cross section measurements. Although many parameterizations of the flux of solar energetic particles give acceptable fits to the experimental data for 74275, we prefer a best fit obtained for 10Be and 26Al alone, which incorporates an erosion rate of ∼2 mm/Ma, a rigidity of 100 MV, and a 4π flux of protons with energies greater than 10 MeV of 89 cm−2 s−1. For 41Ca alone, the corresponding values are 2 mm/Ma, 80 MV, and 198 cm−2 s−1. The differences between the two sets of parameters may reflect uncertainties in the calculations of 41Ca production or a secular change in the solar cosmic ray flux. Calculations for a slab and for a hemispherical knob with a radius of 23 cm yield similar results. © 1998 Elsevier Science Ltd.
59Ni production rates in mesosiderites measured with AMS
(Wiley, 1993-07-01) Fink, D; Tuniz, C; Herzog, G; Albrecht, A; Fifield, LK; Allen, GL; Paul, M
The cosmogenic radionuclide 59 Ni(t1/2=76ka) has great potential as a monitor of thermal neutrons in metal-rich extraterrestrial materials. In deep samples from larger meteoroids (which can support a big neutron flux) containing >1% or so of nickel, thermal neturon capture on 58Ni (delta th=4.6b) is the dominate production mechanism. Near the surface of millimeter-sized bodies production occurs via primary proton, fast neutron, and a reaction channels on Fe, Co, and Ni. We have applied AMS to the measurement of 59Ni activities (see [1] for details) in four samples from the metal phase to f the mesosiderites Estherville (fall,1879) and Budulan(find). The activities range from 1.5 to 3.5 dmp/g-Ni. Related work is described in [2,3]. To discuss neutron fluxes in Budulan, we must correct the measured 59Ni activities for terrestrial age. By using measured 41Ca activities (13-19 dpm/kg-Fe [4]) and a maximum production rate PFe(41Ca), in stony irons of 21dpm/kg-Fe [5] we deduce a maximum terrestrial age of 35 ka. After correction for this terrestrial age and normalization of L-chondrite composition [6], the production rates of 59Ni,PFe(59Ni), range from 5-13 dpm/g-Ni; these values are 2-3x greater than those reported in [7] for large irons and ~10x those for chondrites. Albrecht et al. [4] and Fink et al. [8] present 41Ca data in the silicate and metal phases from the same Estherville and Budulan samples. If thermal neutron production were solely responsible for PFe(59Ni) and PS2(41Ca) (the latter corrected for spalliation of oxidized iron in pyroxene), the thermal neutron fluxes, o, inferred from each nuclide in a sample should be the same. We deduce ratios of o(59Ni)/o(41Ca) that range from 0.75 to 1.65. Differences in epithermal yields can account for only a minor fraction of this variation as the ratio of the total resonant neutron absorption intergrals for 40Ca and 58Ni is within 10% of the ratio of the thermal neutron cross sections alone. A twofold change in Budulan's terrestrial age alters the flux ratio by 10% at most. Like 41Ca[9,10], PFe(59Ni) can be used to estimate shielding depths and lower limits on the preatmospheric radius. Calculations by [11] give a maximum value for PFe(59Ni) of 22 atoms/min/g-Ni at the center of an L chondrite with a radius of 300 g/cm2. The 10Be and 26A1 activities in Estherville [5] and respective semi-empirical production rate formulas [12] set a maximum meteoroid radius of 300 g/cm2. Our measured value for 59Ni implies a lower radius limit of 150 g/cm2 and shielding depths of 60-150g/cm2. Similarly, we suggest a radius of 200< R < 400 g/cm2 and shielding depths from 40-200 g/cm2 for Budalan. We infer that the above samples originated at relatively large depths (except for perhaps Budulan 2428) in meteoroids with preatmospheric radii >30cm, assuming a mesosiderite density of 5.5 g/cm3. Interestingly, those samples (Budulan2357 and Estherville 3311) having 41Ca production rates that indicate a higher degree of shielding have flux rations equal to or less than 1; the other two samples have 41Ca contents typical of near-surface exposure and have ratios o(59Ni)/o(41Ca) larger than unity. This correlation indicates that P59 from fast neutron reactions on 60,61Ni enhances 59Ni production at near-surface regions.
7Be and 10Be concentrations in recent firn and ice at Law Dome, Antarctica
(Elsevier, 2000-10-01) Smith, AM; Fink, D; Child, DP; Levchenko, VA; Morgan, VI; Curran, MAJ; Etheridge, DM; Elliott, G
Over the past three years, the Australian National Tandem for Applied Research (ANTARES) AMS facility at ANSTO has been expanding its sample preparation and measurement capability, particularly for 10Be, 26Al and 36Cl. During this time, ANSTO has continued its collaboration with the AAD and CSIRO Atmospheric Research on the measurement of cosmogenic isotopes from Law Dome, Antarctica. This research program has been supported by the construction of a dedicated geochemistry laboratory for the processing of ice and rock samples for the preparation of AMS targets. Here we present our first results for 10Be concentrations measured in ice cores from three sites at Law Dome and describe the sample processing protocol and aspects of the AMS measurement procedure. These sites are characterised by an eightfold difference in accumulation rate with a common precipitation source. In combination with an established ice chronology, this has enabled some preliminary findings concerning the relationship between the snow accumulation rate and the measured 10Be concentration for Law Dome during recent times. Additionally, we present 7Be and 10Be/7Be measurements made for a few surface snow samples from Law Dome and Australia. © 2000 Elsevier Science B.V.
Accelerator mass spectrometry analyses of environmental radionuclides: sensitivity, precision and standardisation
(Elsevier, 2000-10-01) Hotchkis, MAC; Fink, D; Tuniz, C; Vogt, S
Accelerator Mass Spectrometry (AMS) is the analytical technique of choice for the detection of long-lived radionuclides which cannot be practically analysed with decay counting or conventional mass spectrometry. AMS allows an isotopic sensitivity as low as one part in 1015 for 14C (5.73 ka), 10Be (1.6 Ma), 26Al (720 ka), 36Cl (301 ka), 41Ca (104 ka), 129I (16 Ma) and other long-lived radionuclides occurring in nature at ultra-trace levels. These radionuclides can be used as tracers and chronometers in many disciplines: geology, archaeology, astrophysics, biomedicine and materials science. Low-level decay counting techniques have been developed in the last 40–50 years to detect the concentration of cosmogenic, radiogenic and anthropogenic radionuclides in a variety of specimens. Radioactivity measurements for long-lived radionuclides are made difficult by low counting rates and in some cases the need for complicated radiochemistry procedures and efficient detectors of soft β-particles and low energy x-rays. The sensitivity of AMS is unaffected by the half-life of the isotope being measured, since the atoms not the radiations that result from their decay, are counted directly. Hence, the efficiency of AMS in the detection of long-lived radionuclides is 106–109 times higher than decay counting and the size of the sample required for analysis is reduced accordingly. For example, 14C is being analysed in samples containing as little as 20 μg carbon. There is also a world-wide effort to use AMS for the analysis of rare nuclides of heavy mass, such as actinides, with important applications in safeguards and nuclear waste disposal. Finally, AMS microprobes are being developed for the in-situ analysis of stable isotopes in geological samples, semiconductors and other materials. Unfortunately, the use of AMS is limited by the expensive accelerator technology required, but there are several attempts to develop compact AMS spectrometers at low (⩽0.5 MV) terminal voltages. Recent advances in AMS will be reviewed with highlights from the scientific programs at Lucas Heights and other AMS centres. © 2000 Elsevier Science Ltd.
Accelerator mass spectrometry on SIRIUS: new 6MV spectrometer at ANSTO
(University of Jyväskylä, Finland, 2016-07-03) Wilcken, KM; Fink, D; Hotchkis, MAC; Garton, D; Button, D; Mann, M; Kitchen, R
As a part of Australian Federal Government funding in 2009 to establish a centre for accelerator science a new 6 MV state of the art accelerator – SIRIUS – was purchased. The system is now commissioned and comprises ion sources and beam lines to cater for a wide variety of both IBA and AMS applications. The ion source used for AMS (MC-SNICS) is the latest incarnation followed by 45 degree spherical ESA(R=0.3 m) and double focusing injection magnet (R=1 m, ME=20) prior the accelerator. At the terminal we have a choice of 2 stripper gasses and/or stripper foils. The high-energy spectrometer for AMS consists of a 1.27 m radius analyzing magnet with ME=176, 45 degree ESA (R=3.81m), followed by a switching magnet and 3 beam lines: one with a standard multianode ionization chamber; one with an absorber cell in front of the detector; whereas the third beam line has a time-of- ight detector. Details of the instrument design and performance data for 10Be, 26Al and 36Cl will be presented. © The Authors
Accelerator mass spectrometry on SIRIUS: new 6MV spectrometer at ANSTO
(Elsevier, 2016-07-08) Wilcken, KM; Fink, D; Hotchkis, MAC; Garton, D; Button, D; Mann, M; Kitchen, R
The Centre for Accelerator Science at ANSTO operates four tandem accelerator systems for Accelerator Mass Spectrometry (AMS) and Ion Beam Analysis (IBA). The latest addition to the fleet is SIRIUS, a 6 MV combined IBA and AMS system. Following initial ion beam testing, conditioning and debugging software and hardware, SIRIUS is now commissioned. Details of the instrument design and performance data for 10Be, 26Al and 36Cl are presented.
Accelerator mass spectrometry ultrasensitive analysis for global science
(CRC Press, 1998-03-25) Tuniz, C; Kutschera, W; Fink, D; Herzog, GF; Bird, JR
This extensive undertaking, Accelerator Mass Spectrometry, conducts an elaborate and comprehensive summary of one of the foremost catalysts of progress in scientific research. Accelerator mass spectrometry (AMS), an innovative analytical technique, measures rare atoms at unprecedented levels of sensitivity, revolutionizing the science of radiocarbon dating and accessing new natural radioisotopes as environmental tracers and chronometers. This book demonstrates how AMS is applied in the studies of extraterrestrial materials, the earth sciences, the future of the global environment, and the history of mankind. This compendium also highlights the significant impact of AMS on several fields of scientific investigation, spurring remarkable studies in global climate change, ancient artifacts, pollution, nuclear safeguards, geochronology, and materials characterization. The myriad of sample types and variety of applications in this examination include: Meteorites from Mars Ancient air trapped in Antarctic ice The Shroud of Turin The dating of human bones The colonization of the Americas and Australia Ancient rock art The crown of Charlemagne Cancerogenic effects of cooked meat The consequences of the Chernobyl accident The role of aluminum in Alzheimer's Disease This unique edition has compiled the diverse set of scientific literature into a single volume, suitable as a text or resource on the major AMS-related outcomes, issues, and methods.

Browsing by Author "Fink, D"

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