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Browsing by Author "Drysdale, RN"

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A 1,000 year rainfall record for SE Australia using speleothem hydrological proxies
(Geological Society of Australia, 2010-07-04) McDonald, J; Drysdale, RN; Hodge, E; Hua, Q; Fischer, MJ; Treble, PC; Greig, A; Hellstrom, JC
Cave drip water studies at Wombeyan Caves (34°19’S, 149°59’E) demonstrated a marked hydrochemical response to wet/dry (McDonald et al., 2004; 2007). Three 20th Century coeval active speleothems (WM4, WM6 and WM20) were geochemically analysed and changes in trace element and stable isotope values were related to the instrumental record. These climate‐geochemical relationships were interpolated to two longrecord speleothems (WM7 and WM9) which grew deeper within the same cave system. Two major difficulties were encountered. Unlike other sub‐annual/annual climate records derived from speleothems using trace elements (Treble et al., 2003; Johnson et al., 2006); stable isotopes (Treble et al., 2005; Johnson et al., 2006) and annual laminae (Borsato et al., 2007) where annual cycles were shown to be consistent, at Wombeyan frequent droughts perturb predicted rainfall patterns and rainfall variability is high. Here, droughts can span several years, or extend over winter, diminishing or obliterating the expected winter recharge signal. Alternatively, wet summers can sustain ‘unseasonal’ high discharge and lessen the expected prior calcite precipitation (PCP) signal. Thus an annual wet/dry geochemical signal is often absent. Secondly, due to the young age of the speleothems and very low uranium concentrations (~10 ppb) the use of U‐series disequilibrium dating was ineffective to produce a robust chronology. Trace element cycle counting only gave the minimum age due to the non‐expression of many cycles. The 14C bomb pulse was successfully defined in two modern stalagmites (WM4 and WM6) and maximum 14‐C activity was around 134 per cent modern carbon (pMC) for both speleothems, indicating rapid transfer of 14‐C from atmosphere, to soil, to drip water during the bomb‐pulse period. A dampened 14C bomb pulse was detected in WM7 (where pMCmax was 112 per cent modern carbon) reflecting the greater degree of mixing within the thicker bedrock. Carbon‐14 AMS analyses were utilised together with trace element cycle counting to obtain preliminary chronological control. Despite these difficulties, palaeohydrological records using multiple proxies: Mg/Ca (aridity), P and Y (wet), δ18O (dominant air mass and rainfall amount signals), and based on 14C ages were constructed for the longerrecord, slower growing stalagmites. Over the last 1,000 years there have been several sustained episodes of wet/arid or highly variable phases. A sustained wet phase occurred ~ 900–1300 AD and followed by ~ 200 years of highly variable wet/dry conditions. From ~ 1500 to 1800 AD a dry phase is indicated. The last 150 years support a drying phase, but the negative IPO (1944–1978 [wettest period in 20thC]) is not indicated by a negative anomaly and further, sustained positive δ18O anomalies in this period suggest that other factors maybe influencing this part of the record (temperature?). The δ18O record indicates changing frequency from ~ centennial to pentadecadal time‐scales in the longer‐time scale oscillations. Within the longer‐time scale oscillations, higher resolution (~ 2–5 years) variability is evident replicating the trend shown by modern annually resolved stalagmites at this site.
A 1,500 year south Australian rainfall record based on speleothem hydrological proxies
(AMOS National Conference, 2013-02-11) McDonald, J; Drysdale, RN; Hua, Q; Hodge, E; Treble, PC; Greig, A; Fallon, SJ; Lee, S; Hellstrom, JC
Cave drip water studies at Wombeyan Caves (34°19’S, 149°59’E) demonstrated a marked hydrochemical response to wet/dry phases (McDonald Et al. 2004; 2007). Geochemical Variations in three 20th Century coeval active Speleothems were able to be linked to the instrumental record. Subsequently geochemical relationships were investigated in a long record speleothem(WM7) which grew deeper within the same cave system. Obtaining a robust chronology proved to be challenging, due to the young age of the speleothem and very low uranium concentrations (~10 ppb) the use of U‚Aeseries disequilibrium dating was ineffective to produce a robust chronology. Chronology for WM7 was based on a dense sequence of DCF corrected ages using three different age-‐depth models: Clam (Classical method), and Bacon and OxCal (Bayesian statistical approach) (Hua et al. 2012).The new chronology indicated that WM7 began growth around 4400 cal BP(171 mm). However, since sampling from 0-‐50mm was most intensive, the model is based on this part of the stalagmite and indicates that the top 50 mm of WM7 grew during the past 1360 and 1740 years. An aridity index based on Sr,P, Y, La, and Ba shows that over the last 1,500 years several sustained episodes of wet/arid and otherwise variable phases have occurred. Two sustained wet phases ~ 700-‐880 AD and ~ 900-‐ 1250 AD were followed by ~ 400 years of variable wet/dry conditions, although from ~1300 to 1600 AD a drying trend is indicated, but punctuated by several wetter episodes. The last 200 years indicate sustained drying phases. The OE￥13C record is anomalous from ~ 1880 to present and attributed to the stalagmite’s recording of increasing contribution of fossil fuel to CO2 concentrations. Within the longer-‐time scale oscillations, higher resolution (~ 2-‐5 years) variability is evident, replicating the trend shown by modern annually resolved stalagmites at this site.
Assessment of climatic influences on 14C activity in a Holocene stalagmite from Flores, Indonesia
(University of Newcastle, 2010-06-30) Griffiths, ML; Drysdale, RN; Hua, Q; Hellstrom, JC; Frisia, S; Gagan, MK; Zhao, JX; Ayliffe, LK
In the last decade, a number of speleothem studies have used radiocarbon dating to address a range of paleoclimate problems. These have included the use of the bomb pulse to anchor chronologies over the last 60 years (Mattey et al 2008), the combining of U-series and radiocarbon measurements to improve the radiocarbon calibration curve (Beck et al. 2001), and linking atmospheric radiocarbon variations with climate changes (McDermott et al. 2008). Central to a number of these studies is how to constrain, or interpret variations in, the amount of radioactively dead carbon (i.e. the dead carbon fraction, or DCF) that contributes to a speleothem radiocarbon measurement. In this study, we use radiocarbon measurements, stable isotope and trace element geochemistry, and U-series ages to examine DCH variations between 2.4 and 2.8 ka in a previously studied (Griffiths et al. 2009; 2010) speleothem from Liang Luar, Flores, Indonesia.
Characterising the expression of sub-millennial scale climate events in western Europe during the early last glacial period using multi-proxy speleothem records
(Australasian Quaternary Association Inc., 2022-12-06) Corrick, E; Drysdale, RN; Hellstrom, JC; Couchoud, I; Wong, HKY; Didier, C; Hai, C; Jaillet, S; Tocino, S
Past abrupt climate changes act as critical analogues for understanding how the climate system may respond to future abrupt changes. One of the best examples of naturally occurring abrupt climate change is the series of millennial-scale Dansgaard-Oeschger (D-O) events that took place during the last glacial period (115,000 – 11,500 years ago). D-O events are clearly recorded in ice-cores from Greenland, with coincident climate changes detected in marine and terrestrial records spanning a range of climate zones. Greenland ice cores also record shorter-lived ‘sub-millennial’ scale events that occur within the main D-O event sequence, particularly during the early last glacial period. To what extent these sub-millennial events were expressed outside of Greenland is currently poorly understood. Here we characterise the response to sub-millennial scale climate changes in western Europe using five multi-proxy (δ18O, δ13C, Mg and Sr) speleothem records from Saint-Marcel and Orgnac Caves, France, that collectively span 127 – 87 kyr BP. The replicated speleothem records clearly preserve both millennial D-O events and sub-millennial events, demonstrating the strong coupling between the climate of south-east France and the North Atlantic across both millennial and sub-millennial timescales. Interestingly, the multiproxy record reveals a decoupling between broad temperature (indicated by δ13C) and precipitation changes (indicated by δ18O) during some of these sub-millennial scale events. This suggests that climate teleconnections operating during sub-millennial events were in some ways different to those during the stronger millennial-scale D-O events.
Clumped isotope analysis of Central Australian carbonates: a potential palaeoclimate proxy for Australia’s arid interior
(American Geophysical Union (AGU), 2022-12-13) Nixon, F; Tyler, JJ; Priestley, SC; Cohen, TJ; Klaebe, RM; Crossey, LJ; Karlstrom, KE; Polak, VJ; Asmerom, Y; Love, AJ; Hua, Q; Wade, B; Pollard, T; Drysdale, RN; Hall, PA
Quantitative records of past temperature variability in arid environments are crucial for validating climate models and their ability to capture the full range of the Earth’s climatic regions. However, arid zone temperature reconstructions are rare, particularly in the Southern Hemisphere, including Australia. The clumped isotope thermometer provides a novel approach to potentially address this demand by allowing the estimation of carbonate precipitation temperature independent of environmental water isotopic composition. Two types of carbonate materials offer potential for clumped isotope temperature reconstructions in arid central Australia: fossil mollusk shells deposited within the shoreline sediments of now dry lakes, and tufa deposits formed in mound springs fed by continuous discharge of Great Artesian Basin groundwater. Here we present preliminary clumped isotope analyses from tufa and shell samples from central Australia. We also discuss the use of micro-XRF scanning and XRD to evaluate sample suitability for both clumped isotope analysis and U-series dating. Air temperatures inferred from tufa Δ47 measurements suggest mean annual air temperatures (MAAT) ~5°C cooler than present between 12-9 ka, which supports palaeoclimate model based estimates for central Australia. Average air temperatures inferred from mollusk shells indicate MAAT at least 15°C cooler than present during 70-35 ka, suggesting a larger MAAT reduction than previously estimated. Carbonate δ18O appears to have been largely driven by changes in environmental water δ18O for lakes but not for mound springs, reflecting different hydrological controls on the two water sources. Agreement between temperatures and palaeoclimate models suggest clumped isotope analysis may function as a valuable quantitative palaeotemperature proxy in central Australia. Analysis of additional tufa and shell samples along with an investigation of the genesis of different tufa is ongoing.
Clumped isotope analysis of central Australian carbonates: a potential palaeoclimate proxy for Australia’s arid interior
(Australasian Quaternary Association Inc., 2022-12-06) Nixon, F; Tyler, JJ; Priestley, SC; Cohen, TJ; Klaebe, RM; Crossey, LJ; Karlstrom, KE; Polyak, VJ; Asmerom, Y; Love, A; Hua, Q; Wade, B; Pollard, T; Drysdale, RN; Hall, PA
Quantitative records of past temperature variability in arid environments are crucial for validating climate models and their ability to capture the full range of the Earth’s climatic regions. However, arid zone temperature reconstructions are rare, particularly in the Southern Hemisphere, including Australia. The clumped isotope thermometer provides a novel approach to potentially address this demand by allowing the estimation of carbonate precipitation temperature independent of environmental water isotopic composition. Two types of carbonate materials offer potential for clumped isotope temperature reconstructions in arid central Australia: fossil mollusk shells deposited within the shoreline sediments of now dry lakes, and tufa deposits formed in mound springs fed by continuous discharge of Great Artesian Basin groundwater. Here we present preliminary clumped isotope analyses from tufa and shell samples from central Australia. We also discuss the use of micro-XRF scanning and XRD to evaluate sample suitability for both clumped isotope analysis and U-series dating. Air temperatures inferred from tufa Δ47 measurements suggest mean annual air temperatures (MAAT) ~5°C cooler than present between 12-9 ka, which supports palaeoclimate model based estimates for central Australia. Average air temperatures inferred from mollusk shells indicate MAAT at least 15°C cooler than present during 70-35 ka, suggesting a larger MAAT reduction than previously estimated. Carbonate δ18O appears to have been largely driven by changes in environmental water δ18O for lakes but not for mound springs, reflecting different hydrological controls on the two water sources. Agreement between temperatures and palaeoclimate models suggest clumped isotope analysis may function as a valuable quantitative palaeotemperature proxy in central Australia. Analysis of additional tufa and shell samples along with an investigation of the genesis of different tufa is ongoing.
Environmental change in the Adriatic region over the last 365 kyr from episodic deposition of Modrič Cave (Croatia) speleothems
(International Union for Quaternary Research (INQUA), 2019-07-25) Surić, M; Lončarić, R; Columbu, A; Bajo, P; Lončar, N; Drysdale, RN; Hellstrom, JC
The Adriatic Sea, as the northernmost and practically landlocked part of the Mediterranean Sea, is influenced by both Atlantic and Mediterranean air masses, so the isotopic records from coastal cave speleothems are expected to reveal local and regional responses to global climate changes on that bordering region. In this study we present a 365-kyr long composite isotopic record of three speleothems from Modrič Cave located 120 m from the shoreline on the central part of the eastern Adriatic coast. Results of a 4-year monitoring program of the surface and cave microclimate, rain and drip water stable isotope composition and rain and drip intensities, show cave air temperature variations within 1 °C, a relative humidity of 100%, dripwater O and H stable isotopic composition (range 0.4‰) very well buffered against the seasonal rainfall range (6.8‰). Such conditions enable calcite deposition without strong kinetic isotopic disequilibrium effects, as validated by Hendy tests, and give us confidence that the isotopic signal is faithfully recording climate changes. All three speleothems (MOD-31, MOD-32, MOD-33) were active, collected from their growth position, so Holocene signals can be traced in all of them. Within their older parts, U-Th dating reveals the following growth periods: MOD-31 from MIS 10 to MIS 7, MOD-32 from MIS 4 to MIS 2, and MOD-33 from MIS 6 to MIS 5. Relatively large δ18O and δ13C ranges (-8.16‰ – -2.97‰ and -13.11‰ – -1.00‰, respectively) indicate significant environmental changes whose comparison with stable isotope time series of adjacent speleothem records and other regional proxies provides the longest eastern Adriatic speleothem-based record. © 2019 The Authors.
Evidence for Holocene changes in Australian-Indonesian monsoon rainfall from stalagmite trace element and stable isotope ratios
(Elsevier, 2010-03-15) Griffiths, ML; Drysdale, RN; Gagan, MK; Frisia, S; Zhao, JX; Ayliffe, LK; Hantoro, WS; Hellstrom, JC; Fischer, MJ; Feng, YX; Suwargadi, BW
Trace element and stable isotope ratios from an active stalagmite (LR06-B1) recovered from Liang Luar Cave on the island of Flores (eastern Indonesia) are used to reconstruct the position of the austral summer inter-tropical convergence zone and Australian-Indonesian summer monsoon variability during the Holocene. Uranium-series dating of the stalagmite shows that it commenced growth 12,640 years ago , with hiatuses spanning 8,560 to 6,420 and 3,670 to 2,780 years ago. Stalagmite Mg/Ca and Sr/Ca ratios correlate significantly with one another, and with δ18O and δ13C, throughout the record. This suggests that the Mg/Ca and Sr/Ca ratios are dominated by prior calcite precipitation, a process whereby degassing in the vadose zone during periods of low recharge causes deposition of calcite and disproportionate loss of Ca2+ ions (relative to Mg2+ and Sr2+) ‘upstream’ of the stalagmite. The degree of initial 234U/238U disequilibrium also appears to have been controlled by recharge to the overlying aquifer. Together with the Mg/Ca, Sr/Ca, and δ18O values, the initial uranium isotope activity ratios ([234U/238U]I) imply a generally drier early Holocene, coincident with a lower sea level and lower Southern Hemisphere summer insolation. Comparison of speleothem δ18O time-series from Flores and Borneo shows that they vary in unison for much of the Holocene. However, there is a significant decrease in the Borneo δ18O record ~6,000 to 4,000 years ago that does not occur in the Flores record. This anomaly may be related to a change in the Australian-Indonesian summer monsoon circulation in response to a protracted positive phase of the Indian Ocean Dipole. Under this scenario, stronger upwelling off of western Indonesia would, based on present-day effects, result in reduced summer convective activity over Flores and a subsequent northward shift of the intertropical convergence zone. © 2010, Elsevier Ltd.
A high-resolution record of south-eastern Australian hydroclimate between 30,000 - 10,000 years ago: toward a better understanding of the Australian LGM
(International Union for Quaternary Research (INQUA), 2019-07-29) Falster, G; Tyler, JJ; Grant, K; Tibby, J; Turney, C; Löhr, S; Jacobsen, GE; Kershaw, AP; Kluge, T; Drysdale, RN; Dux, F
Global climate variability during the late Quaternary is commonly framed in terms of the ‘bipolar seesaw’ pattern of asynchronous temperature variations in the northern and southern polar latitudes. However, the terrestrial hydrological response to this pattern in south-eastern Australia is not fully understood, as continuous, high-resolution, well-dated proxy records for the hydrological cycle in the region are sparse. Here we present a well-dated, highly resolved record of moisture balance spanning 30000 – 10000 calendar years before present (30 – 10 ka BP), based on x-ray fluorescence and organic carbon isotope (δ13COM) measurements of a sedimentary sequence from Lake Surprise in south-eastern Australia. The data provide a locally coherent record of the hydrological cycle (Fig. 2). Elevated Si (reflecting windblown quartz and clays), and relatively high δ13COM, indicate an extended period of relative aridity between 28 – 17.5 ka BP, interrupted by millennial-scale episodes of decreased Si and δ13COM, suggesting increased moisture balance. Peak aridity was reached between 21 and 17.5 ka BP, possibly representing the expression of the global Last Glacial Maximum. This was followed by a rapid deglacial shift to low Si and δ13COM at 17.5 ka BP, indicative of wetter conditions. We find that these changes are broadly coeval with similarly high-resolution records from south-eastern Australia and New Zealand. We also supplement our high-resolution record with discrete clumped isotope measurements on freshwater gastropods from Blanche Cave, also in south-eastern Australia. Temperatures either side of the Last Glacial Maximum were slightly cooler than those of the modern day, with the hint of a decrease from 40 to 30 ka BP. We did not find gastropods within the 28-17.5 ka BP interval in this cave, but identify this as a period for urgent attention. Together, our analyses suggest that drivers of the regional hydrological cycle have varied on multi-millennial time scales, in response to major shifts in global atmosphere-ocean dynamics during the last glacial-interglacial transition. Southern Ocean processes were the dominant control on hydroclimate during glacial times, via a strong influence of cold sea surface temperatures on moisture uptake and delivery onshore. Following the last deglaciation, the southward migration of cold Southern Ocean fronts likely resulted in the establishment of conditions more like those of the present day. These conclusions will be tested in future work, focused on quantitative rainfall estimates from clumped isotope of land snail shells. Figure 1. Selected data from the Lake Surprise record: a) Bulk sediment carbon isotope ratios (δ13COM), interpreted to reflect plant moisture stress; b) First principal component (PC1) of the calibrated scanning XRF dataset, interpreted to reflect aeolian deposition of Si. Arrows indicate periods of increased effective moisture within the relatively arid LGM. Triangles denote 14C age control points.
Human impact on the environment in Western Flores, Indonesia during the late Holocene: identifying agricultural transitions
(18th INQUA Congress, 2011-07-21) St Pierre, E; Zhao, JX; Aplin, K; Drysdale, RN; Golding, SD; Griffiths, ML; Hua, Q
Limestone caves can act as excellent repositories of palaeoenvironmental information and past human activities. This paper presents a multi-proxy record of late Holocene palaeoclimate and palaeoenvironmental change derived from environmental archives in Liang Luar (Steam Cave), western Flores, Indonesia. Liang Luar, located ~1 km from Liang Bua (the discovery site of the hominid species Homo floresiensis), is a ~1.6km long passage with several large chambers and numerous speleothems (stalagmites and stalactites). A palaeoclimate record was compiled using stable carbon and oxygen isotope ratios from a stalagmite precisely dated to 0-1800 yr BP using U/Th dating. The stalagmite isotope record preserves an episode of rapid vegetation change c. 800 yr BP marked by a large shift in carbon and decoupling of the carbon from the oxygen isotopes, and thus thought to be unrelated to climate. Excavated owl pellet deposits in the entrance of Liang Luar dated by 14C AMS on charcoal, reveal continuous sediment deposition from at least 2400 yr BP to the present. The 14C chronology demonstrates a sudden increase in depositional rates at the cave entrance as well as an increase in the abundance of charcoal fragments, at the time of the vegetation change inferred from the stalagmite record. Faunal remains indicate the commensal species Rattus exulans, arrives early in the sequence, while Rattus rattus appears much later. A surprisingly late appearance of two rodents associated with irrigated rice fields, together with a surge in frog remains, indicates wet rice farming was only recently introduced to the area. These paleoenvironmental records act as a basis from which to understand the timing and intensity of human impacts on late Holocene environments in western Flores, and the relationship of this incursion to changing land use patterns. Copyright (c) 2011 INQUA 18
The hydrochemical response of cave drip waters to sub-annual and inter-annual climate variability, Wombeyan Caves, SE Australia
(Elsevier, 2007-10-15) McDonald, J; Drysdale, RN; Hill, DE; Chisari, R; Wong, HKY
A thorough understanding of cave seepage waters is necessary to interpret geochemical variations in speleothem calcite in terms of changing surface climatic conditions at a particular site. Here we present the hydrochemistry of ten cave drip waters from a karst system in SE Australia based on up to 5.5 years of monitoring. Discharge was continuously measured at six sites and manually at the other sites. Dripwater samples were analysed for pH, electrical conductivity, cations and anions at all sites at monthly or more frequent intervals. Each drip possesses a unique chemistry, and not all drip waters responded to antecedent short-term hydrological variations. For example, the hydrochemical behaviour of three adjacent drips at a bedrock depth of 45 m was completely different to that of shallower sites, and was apparently un-related to surface hydrology throughout the investigation. Based on modelled calcite precipitation vectors, prior calcite precipitation was demonstrated at several sites but can only be linked directly to changes in surface recharge at the shallowest sites. At extremely low flow, shallow drip waters accessed a high Mg, Sr and Ba source, thought to be the overlying soil. High-frequency sample collection allows for the calculation of predicted Mg/Ca-calcite and Sr/ Ca-calcite values, highlighting that the sites with the greatest potential to record high-resolution palaeohydrological records are those situated at shallow depth. Longer temporal-resolution palaeohydrological records may be recorded at deeper sites but longer-term monitoring is required to identify probable time scales. Inherent system non-linearities, dissolution of secondary calcite in pore spaces of the aquifer, changes in the source of trace elements, and the presence of multiple reservoirs confirm the need for the use of multiple speleothems and a multi-proxy approach to gain accurate palaeohydrological records from this site. © 2007, Elsevier Ltd.
Hydrological control on the dead-carbon content of a tropical Holocene speleothem
(Elsevier, 2012-12-01) Griffiths, ML; Fohlmeister, J; Drysdale, RN; Hua, Q; Johnson, KR; Hellstrom, JC; Gagan, MK; Zhao, JX
Over the past decade, a number of speleothem studies have used radiocarbon (14C) to address a range of palaeoclimate problems. These have included the use of the bomb pulse 14C to anchor chronologies over the last 60 years, the combination of U-Th and 14C measurements to improve the radiocarbon age-calibration curve, and linking atmospheric 14C variations with climate change. An issue with a number of these studies is how to constrain, or interpret, variations in the amount of radioactively dead carbon (i.e. the dead carbon fraction, or DCF) that reduces radiocarbon concentrations in speleothems. In this study, we use 14C, stable-isotopes, and trace-elements in a U-Th dated speleothem from Flores, Indonesia, to examine DCF variations and their relationship with above-cave climate over the late Holocene and modern era. A strong association between the DCF and hydrologically-controlled proxy data suggests that more dead carbon was being delivered to the speleothem during periods of higher cave recharge (i.e. lower δ18O, δ13C and Mg/Ca values), and hence stronger summer monsoon. To explore this relationship, we used a geochemical soil-karst model coupled with 14C measurements through the bomb pulse to disentangle the dominant components governing DCF variability in the speleothem. We find that the DCF is primarily controlled by limestone dissolution associated with changes in open- versus closed-system conditions, rather than kinetic fractionation and/or variations in the age spectrum of soil organic matter above the cave. Therefore, we infer that periods of higher rainfall resulted in a higher DCF because the system was in a more closed state, which inhibited carbon isotope exchange between the karst water dissolved inorganic carbon and soil-gas CO2, and ultimately led to a greater contribution of dead carbon from the bedrock. © 2020 Elsevier B.V.
Hydrological influence on the dead carbon fraction in a tropical speleothem during the Younger Dryas and the Last Millennium
(American Geophyical Union, 2015-11-16) Griffiths, ML; Hua, Q; Drysdale, RN; Bajo, P; Jenkins, D; Hellstrom, JC; Johnson, KR; Gagan, MK; Zhao, JX
The number of paleoclimate records derived from speleothems has increased significantly in recent years. In addition, speleothems have been used for calibration of the radiocarbon timescale beyond the range of the tree-ring record. One critical issue for reliable speleothem-based radiocarbon calibration and 14C dating of speleothems is constraining the temporal variations in the radioactively dead carbon (i.e. dead carbon fraction (DCF)) that is incorporated into this archive and to determine the potential mechanisms driving such changes. While some studies have shown insignificant variations in DCF through time and highlighted the potential utility of speleothems to extend/improve the radiocarbon calibration curve, others have reported significant temporal variability in speleothem DCF associated with changes in cave recharge. To further assess the potential hydrological control on speleothem radiocarbon variability, we constructed a new high-resolution DCF record from a speleothem from Flores, Indonesia for two different time periods, the Younger Dryas (YD) chronozone and the Last Millennium. A total of thirty-four 14C analyses (twenty for the YD and fourteen for the Last Millennium) were conducted on pieces of calcite extracted from stalagmite LR06-B1, which was well-dated by ~90 U-Th ages. To better characterize the paleoclimate and environmental changes, high-resolution stable-isotope (δ18O, δ13C) and trace-element (Mg/Ca, Sr/Ca) measurements were also conducted along the same sections of stalagmite. Broad comparison of the DCF record with the hydrologically-controlled proxy data suggests that increases in rainfall were matched by DCF increases. In line with a previous interpretation of DCF variability for the same specimen, but during the time interval 2.4-2.8 cal kyr BP and the post-bomb period, we interpret the DCF during the YD and the Last Millennium to have been primarily controlled by limestone dissolution associated with changes in open- versus closed-system conditions, rather than other potential factors such as kinetic fractionation and/or variations in the age-spectrum of soil organic matter above the cave. American Geophysical Union, Fall Meeting 2015
Increasing Australian-Indonesian monsoon rainfall linked to early Holocene sea-level rise.
(Nature Publishing Group, 2009-09) Griffiths, ML; Drysdale, RN; Gagan, MK; Zhao, JX; Ayliffe, LK; Hellstrom, JC; Hantoro, WS; Frisia, S; Feng, YX; Cartwright, I; Pierre, ES; Fischer, MJ; Suwargadi, BW
The Australian-Indonesian summer monsoon affects rainfall variability and hence terrestrial productivity in the densely populated tropical Indo-Pacific region. It has been proposed that the main control of summer monsoon precipitation on millennial timescales is local insolation(1-3), but unravelling the mechanisms that have influenced monsoon variability and teleconnections has proven difficult, owing to the lack of high-resolution records of past monsoon behaviour. Here we present a precisely dated reconstruction of monsoon rainfall over the past 12,000 years, based on oxygen isotope measurements from two stalagmites collected in southeast Indonesia. We show that the summer monsoon precipitation increased during the Younger Dryas cooling event, when Atlantic meridional overturning circulation was relatively weak(4). Monsoon precipitation intensified even more rapidly from 11,000 to 7,000 years ago, when the Indonesian continental shelf was flooded by global sea-level rise(5-7). We suggest that the intensification during the Younger Dryas cooling was caused by enhanced winter monsoon outflow from Asia and a related southward migration of the intertropical convergence zone(8). However, the early Holocene intensification of monsoon precipitation was driven by sea-level rise, which increased the supply of moisture to the Indonesian archipelago. © 2009, Nature Publishing Group.
Indo-Pacific hydroclimate over the past millennium and links with global climate variability
(American Geophysical Union, 2016-01-01) Griffiths, ML; Drysdale, RN; Kimbrough, AK; Hua, Q; Johnson, KR; Gagan, MK; Cole, JE; Cook, BI; Zhao, JX; Hellstrom, JC; Hantoro, WS
The El Niño-Southern Oscillation (ENSO) and Interdecadal Pacific Oscillation (IPO) are the dominant modes of hydroclimate variability in the tropical Pacific and have far-reaching impacts on Earth’s climate. Experiments combining instrumental records with climate-model simulations have highlighted the dominant role of the Pacific Walker circulation in shaping recent trends in global temperatures (Kosaka and Xie, 2013, 2016). However, the paucity of high-resolution terrestrial paleoclimate records of deep atmospheric convection over the Indo-Pacific Warm Pool (IPWP) precludes a comprehensive assessment as to role of the tropical Pacific in modulating radiative-forced shifts in global temperature on multidecadal to centennial timescales. Here we present a suite of new high-resolution oxygen-isotope records from Indo-Pacific speleothems, which, based on modern rainfall and cave drip-water monitoring studies, along with trace element (Mg/Ca, Sr/Ca) analyses, are interpreted to reflect changes in Australasian monsoon variability during the Common Era (C.E.). Our results reveal a protracted decline in southern Indonesian monsoon rainfall between ~1000-1400 C.E. but stronger between ~1500-1900 C.E. These centennial-scale patterns over southern Indonesia are consistent with other proxy records from the region but anti-phased with records from India and China, supporting the paradigm that Northern Hemisphere cooling increased the interhemispheric thermal gradient, displacing the Australasian ITCZ southward. However, our findings are also compatible with a recent synthesis of paleohydrologic records for the Australasian monsoon region, which, collectively, suggest that rather than moving southward during the LIA, the latitudinal range of monsoon-ITCZ migration probably contracted equatorward (Yan et al., 2015). This proposed LIA ITCZ contraction likely occurred in parallel with a strengthening of the Walker circulation (as indicated through comparison with our hydroclimate records from the central-eastern equatorial Pacific Ocean and western Indian Ocean, and eastern Australia), and thus, the tropical Pacific may have played a critical role in amplifying the radiative-forced global cooling already underway. © 2016. American Geophysical Union
An investigation of the climatic influences on 14C activity in a Holocene stalagmite from Flores, Indonesia
(18th INQUA Congress, 2011-07-21) Griffiths, ML; Drysdale, RN; Hua, Q; Hellstrom, JC; Frisia, S; Gagan, MK; Zhao, JX; Fischer, MJ; Ayliffe, LK
Over the past decade, a number of speleothem studies have used radiocarbon dating to address a range of palaeoclimate problems. These have included the use of the bomb pulse to anchor chronologies over the last 60 years, the combining of U-series and radiocarbon measurements to improve the radiocarbon calibration curve, and linking atmospheric radiocarbon variations with climate changes. Central to a number of these studies is how to constrain, or interpret variations in, the amount of radioactively dead carbon (i.e. the dead carbon fraction, or DCF) that contributes to a speleothem radiocarbon measurement. In this study, we use radiocarbon measurements, stable-isotope and trace-element geochemistry, and U-series ages from a previously studied speleothem from Flores, Indonesia, to examine DCF variations and its relationship with above-cave climate over the late-Holocene to modern interval. A strong association between the DCF and other hydrologically controlled proxy data clearly shows that more dead carbon is being delivered to the speleothem during periods of higher cave recharge (i.e. lower ?18O, ?13C and Mg/Ca values) and hence a stronger summer monsoon. One possible explanation is a higher contribution from the bedrock under such conditions. Although one might expect a concurrent increase in stable carbon isotope values as DCF increases (not observed here), it is possible that such an increase in ?13C may be more than offset by the effect of increased recharge on the rate of carbon dioxide degassing. But, a higher proportion of bedrock carbon is not the only possible explanation: when the monsoon is stronger, a greater proportion of less mobile ‘older carbon’ may be leached from the soil thus diluting the ‘younger carbon’ fraction. This would produce an ‘apparent’ increase in DCF. Copyright (c) 2011 INQUA 18
Last Glacial pluvial periods evident in subaqueous speleothems from Australia’s southern arid-margin
(Australasian Quaternary Association Inc., 2022-12-06) Gould-Whaley, C; Drysdale, RN; May, JH; Hellstrom, JC; Treble, PC; Grieg, A; Cheng, H; Buswell, C
Archives from Kati Thanda (Lake Eyre) basin indicate at least three distinct periods of lake filling during the Last Glacial Period. The headwaters of the megalake lie as far north as -19 °, therefore filling events are indicative of increased intensity of the Indo-Australian Summer Monsoon (IASM). However, due to the nature of unconsolidated materials, these archives are limited in how precisely they can constrain the timing of Last Glacial pluvial periods, and they cannot capture millennial-scale climate variability. Speleothems from Mairs Cave (Flinders Ranges, South Australia), present an opportunity to address these issues. The cave lies on the boundary between the arid and semi-arid regions and currently receives rainfall from both the Southern Hemisphere Westerly Winds (SHWW) and the IASM. The cave contains pendulites: stalactites with an external overgrowth of subaqueously precipitated calcite. The stalactites were initially submerged ~ 89 ka by rising groundwaters, which flooded the cave. From that point forward, the pendulites grew subaqueously during periods of regional groundwater recharge. Preliminary findings suggest periods of subaqueous growth align with higher Southern Hemisphere summer insolation, suggesting the site received enhanced tropical rainfall due to moisture delivery from the IASM. Growth rate and magnesium concentrations both appear to be responsive to millennial-scale climate change, exhibiting increases during both Heinrich events and the cold limbs of Dansgaard-Oeschger events. This is consistent with increased delivery of tropical moisture due to southerly incursions of the IASM. The study site lies near the intersection of two ‘superhighways’ of early human expansion proposed by Crabtree et al. (2021). The cave is also 200 km directly south of the Warratyi shelter, one of the earliest sites of human occupation in southern-central Australia. Therefore, the palaeoclimate record to emerge from this research could potentially provide a more detailed climatic contextualisation for this period of human history.
Magnesium in subaqueous speleothems as a potential palaeotemperature proxy
(Springer Nature, 2020-10-06) Drysdale, RN; Couchoud, I; Zanchetta, G; Isola, I; Regattieri, E; Hellstrom, JC; Govin, A; Tzedakis, PC; Ireland, T; Corrick, E; Grieg, A; Wong, HKY; Piccini, L; Holden, PJ; Woodhead, JD
Few palaeoclimate archives beyond the polar regions preserve continuous and datable palaeotemperature proxy time series over multiple glacial-interglacial cycles. This hampers efforts to develop a more coherent picture of global patterns of past temperatures. Here we show that Mg concentrations in a subaqueous speleothem from an Italian cave track regional sea-surface temperatures over the last 350,000 years. The Mg shows higher values during warm climate intervals and converse patterns during cold climate stages. In contrast to previous studies, this implicates temperature, not rainfall, as the principal driver of Mg variability. The depositional setting of the speleothem gives rise to Mg partition coefficients that are more temperature dependent than other calcites, enabling the effect of temperature change on Mg partitioning to greatly exceed the effects of changes in source-water Mg/Ca. Subaqueous speleothems from similar deep-cave environments should be capable of providing palaeotemperature information over multiple glacial-interglacial cycles. © 2020 The Author(s)
A palaeorainfall record from Central Pacific over the last millennia from speleothems: preliminary results
(International Union For Quaternary Research (INQUA), 2014-07-07) Couchoud, I; Drysdale, RN; Hellstrom, JC; Hua, Q; Spötl, C; Etienne, S
The South Pacific Convergence Zone (SPCZ) is a major feature of the South Pacific basin. Its position and activity fluctuate seasonally and at interannual and decadal timescales under the influence of ENSO and the IPO, driving changes in temperature and precipitation in the region. Zonal SPCZ events have also been shown to be associated to cyclogenesis in the Central Pacific, inducing serious hazards for the islands and populations of French Polynesia1. The reconstruction of past SPCZ position and intensity for pre-industrial periods could help to understand its dynamics and improve models aimed at predicting its evolution in a context of global change but long-term, highly resolved and chronologically well-constrained archives of palaeoclimate from the tropical South and Central Pacific are scarce. To address this issue, we collected speleothems from caves located on the uplifted atoll of Rurutu, in the Australes archipelago at the eastern part of the SPCZ. We present preliminary speleothem proxy data of regional palaeohydrology covering the last few millennia.
Paleoclimate studies and natural-resource management in the Murray-Darling Basin I: past, present and future climates
(Taylor & Francis, 2013-06-19) Mills, K; Gell, PA; Hesse, PP; Jones, R; Kershaw, P; Drysdale, RN; McDonald, J
This paper provides an incisive review of paleoclimate science and its relevance to natural-resource management within the Murray-Darling Basin (MDB). The drought of 1997–2010 focussed scientific, public and media attention on intrinsic climate variability and the confounding effect of human activity, especially in terms of water-resource management. Many policy and research reviews make statements about future planning with little consideration of climate change and without useful actionable knowledge. In order to understand future climate changes, modellers need, and demand, better paleoclimate data to constrain their model projections. Here, we present an insight into a number of existing long-term paleoclimate studies relevant to the MDB. Past records of climate, in response to orbital forcing (glacial–interglacial cycles) are found within, and immediately outside, the MDB. High-resolution temperature records, spanning the last 105 years, exist from floodplains and cave speleothems, as well as evidence from lakes and their associated lunettes. More recently, historical climate records show major changes in relation to El Niño–Southern Oscillation cycles and decadal shifts in rainfall regimes. A considerable body of research currently exists on the past climates of southeastern Australia but, this has not been collated and validated over large spatial scales. It is clear that a number of knowledge gaps still exist, and there is a pressing need for the establishment of new paleoclimatic research within the MDB catchment and within adjacent, sensitive catchments if past climate science is to fulfil its potential to provide policy-relevant information to natural-resource management into the future. © 2013, Taylor & Francis.

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