Superfast proton diffusion achieved in a plasma-polymerized fuel-cell membrane

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dc.contributor.authorPeterson, VKen_AU
dc.contributor.authorCorr, CSen_AU
dc.contributor.authorBoswell, RWen_AU
dc.contributor.authorIzaola, Zen_AU
dc.contributor.authorKearley, GJen_AU
dc.date.accessioned2013-09-19T01:17:21Zen_AU
dc.date.available2013-09-19T01:17:21Zen_AU
dc.date.issued2013-03-07en_AU
dc.date.statistics2013-09-19en_AU
dc.description.abstractWe measure superfast proton diffusion in a proton-exchange membrane (PEM) produced by plasma polymerization. The proton self-diffusion is measured in water-saturated PEMs from the proton autocorrelation function obtained from quasielastic neutron scattering (QENS). 41(3)% of protons in the plasma-produced membrane diffuse at a rate that is an order of magnitude faster than that measured in the commercially available membrane, Nafion, and this is achieved in low hydration conditions. Both molecular dynamic simulations and experimental results are consistent with an assisted superfast diffusion process that may open the way to more powerful fuel cells. © 2013, American Chemical Society.en_AU
dc.identifier.citationPeterson, V. K., Corr, C. S., Boswell, R. W., Izaola, Z., & Kearley, G. J. (2013). Superfast proton diffusion achieved in a plasma-polymerized fuel-cell membrane. Journal of Physical Chemistry C, 117 (9), 4351-4357. doi:10.1021/jp309259ken_AU
dc.identifier.govdoc5163en_AU
dc.identifier.issn1932-7447en_AU
dc.identifier.issue9en_AU
dc.identifier.journaltitleJournal of Physical Chemistry Cen_AU
dc.identifier.pagination4351-4357en_AU
dc.identifier.urihttp://dx.doi.org/10.1021/jp309259ken_AU
dc.identifier.urihttp://apo.ansto.gov.au/dspace/handle/10238/4721en_AU
dc.identifier.volume117en_AU
dc.language.isoenen_AU
dc.publisherAmerican Chemical Societyen_AU
dc.subjectDynamicsen_AU
dc.subjectProtonsen_AU
dc.subjectPlasmaen_AU
dc.subjectMembranesen_AU
dc.subjectNeutronsen_AU
dc.subjectScatteringen_AU
dc.titleSuperfast proton diffusion achieved in a plasma-polymerized fuel-cell membraneen_AU
dc.typeJournal Articleen_AU
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